1Sciences de l'Univers au CERFACS, URA1875, CERFACS/CNRS, Toulouse, France
2Météo France, Toulouse, France
3Deutsches Zentrum für Luft- und Raumfahrt (DLR), Institut für Physik der Atmosphäre, Oberpfaffenhofen, Germany
Received: 07 Dec 2010 – Discussion started: 19 Jan 2011
Abstract. An important issue in the evaluation of the environmental impact of emissions from concentrated sources such as transport modes, is to understand how processes occurring at the scales of exhaust plumes can influence the physical and chemical state of the atmosphere at regional and global scales. Indeed, three-dimensional global circulation models or chemistry transport models generally assume that emissions are instantaneously diluted into large-scale grid boxes, which may lead, for example, to overpredict the efficiency of NOx to produce ozone. In recent times, various methods have been developed to incorporate parameterizations of plume processes into global models that are based e.g. on correcting the original emission indexes or on introducing "subgrid" reaction rates in the models. This paper provides a review of the techniques proposed so far in the literature to account for local conversion of emissions in the plume, as well as the implementation of these techniques into atmospheric codes.
Revised: 25 Jun 2011 – Accepted: 28 Jul 2011 – Published: 05 Aug 2011
Paoli, R., Cariolle, D., and Sausen, R.: Review of effective emissions modeling and computation, Geosci. Model Dev., 4, 643-667, doi:10.5194/gmd-4-643-2011, 2011.