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Geoscientific Model Development An interactive open-access journal of the European Geosciences Union
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GMD | Articles | Volume 11, issue 3
Geosci. Model Dev., 11, 1115–1131, 2018
https://doi.org/10.5194/gmd-11-1115-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue: The Modular Earth Submodel System (MESSy) (ACP/GMD inter-journal...

Geosci. Model Dev., 11, 1115–1131, 2018
https://doi.org/10.5194/gmd-11-1115-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 3.0 License.

Development and technical paper 28 Mar 2018

Development and technical paper | 28 Mar 2018

Polar boundary layer bromine explosion and ozone depletion events in the chemistry–climate model EMAC v2.52: implementation and evaluation of AirSnow algorithm

Stefanie Falk and Björn-Martin Sinnhuber
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Revised manuscript under review for GMD
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Brominated VSLS and their influence on ozone under a changing climate
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Cited articles  
Abbatt, J. P. D., Thomas, J. L., Abrahamsson, K., Boxe, C., Granfors, A., Jones, A. E., King, M. D., Saiz-Lopez, A., Shepson, P. B., Sodeau, J., Toohey, D. W., Toubin, C., von Glasow, R., Wren, S. N., and Yang, X.: Halogen activation via interactions with environmental ice and snow in the polar lower troposphere and other regions, Atmos. Chem. Phys., 12, 6237–6271, https://doi.org/10.5194/acp-12-6237-2012, 2012. a, b, c
Adams, J. W., Holmes, N. S., and Crowley, J. N.: Uptake and reaction of HOBr on frozen and dry NaCl/NaBr surfaces between 253 and 233 K, Atmos. Chem. Phys., 2, 79–91, https://doi.org/10.5194/acp-2-79-2002, 2002. a
Barrie, L. A., Bottenheim, J. W., Schnell, R. C., Crutzen, P. J., and Rasmussen, R. A.: Ozone destruction and photochemical reactions at polar sunrise in the lower Arctic atmosphere, Nature, 334, 138–141, https://doi.org/10.1038/334138a0, 1988. a
Bottenheim, J. W., Gallant, A. G., and Brice, K. A.: Measutements of NOy Species and O-3 at 82-Degrees-N Latitude, Geophys. Res. Lett., 13, 113–116, https://doi.org/10.1029/GL013i002p00113, 1986. a
Bottenheim, J. W., Fuentes, J. D., Tarasick, D. W., and Anlauf, K. G.: Ozone in the Arctic lower troposphere during winter and spring 2000 (ALERT2000), Atmos. Environ., 36, 2535–2544, https://doi.org/10.1016/S1352-2310(02)00121-8, 2002. a
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Ozone depletion events (ODEs) in the polar boundary layer are observed frequently in spring. ODEs serve as a source of tropospheric BrO at high latitudes. A treatment of bromine release and recycling on sea-ice- and snow-covered surfaces is implemented in global chemistry–climate model EMAC based on a scheme of Toyota et al. (2011). Many aspects of bromine enhancement and associated ODEs are reproduced in both polar regions. Further bromine release mechanisms can now be tested in a global model.
Ozone depletion events (ODEs) in the polar boundary layer are observed frequently in spring....
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