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Geoscientific Model Development An interactive open-access journal of the European Geosciences Union
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GMD | Articles | Volume 11, issue 6
Geosci. Model Dev., 11, 2049–2066, 2018
https://doi.org/10.5194/gmd-11-2049-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Special issue: The Modular Earth Submodel System (MESSy) (ACP/GMD inter-journal...

Geosci. Model Dev., 11, 2049–2066, 2018
https://doi.org/10.5194/gmd-11-2049-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Development and technical paper 05 Jun 2018

Development and technical paper | 05 Jun 2018

An advanced method of contributing emissions to short-lived chemical species (OH and HO2): the TAGGING 1.1 submodel based on the Modular Earth Submodel System (MESSy 2.53)

Vanessa S. Rieger et al.

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Butler, T., Lawrence, M., Taraborrelli, D., and Lelieveld, J.: Multi-day ozone production potential of volatile organic compounds calculated with a tagging approach, Atmos. Environ., 45, 4082–4090, https://doi.org/10.1016/j.atmosenv.2011.03.040, 2011. a
Clappier, A., Belis, C. A., Pernigotti, D., and Thunis, P.: Source apportionment and sensitivity analysis: two methodologies with two different purposes, Geosci. Model Dev., 10, 4245–4256, https://doi.org/10.5194/gmd-10-4245-2017, 2017. a
Coates, J. and Butler, T. M.: A comparison of chemical mechanisms using tagged ozone production potential (TOPP) analysis, Atmos. Chem. Phys., 15, 8795–8808, https://doi.org/10.5194/acp-15-8795-2015, 2015. a
Crutzen, P. J. and Schmailzl, U.: Chemical budgets of the stratosphere, Planet. Space Sci., 31, 1009–1032, 1983. a
Deckert, R., Jöckel, P., Grewe, V., Gottschaldt, K.-D., and Hoor, P.: A quasi chemistry-transport model mode for EMAC, Geosci. Model Dev., 4, 195–206, https://doi.org/10.5194/gmd-4-195-2011, 2011. a
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To reduce the climate impact of human activities, it is crucial to attribute changes in atmospheric gases to anthropogenic emissions. We present an advanced method to determine the contribution of emissions to OH and HO2 concentrations. Compared to the former version, it contains the main reactions of the OH and HO2 chemistry in the troposphere and stratosphere, introduces the tagging of the H radical and closes the budget of the sum of all contributions and the total concentration.
To reduce the climate impact of human activities, it is crucial to attribute changes in...
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