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GMD | Articles | Volume 11, issue 8
Geosci. Model Dev., 11, 3369-3389, 2018
https://doi.org/10.5194/gmd-11-3369-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Special issue: The Modular Earth Submodel System (MESSy) (ACP/GMD inter-journal...

Geosci. Model Dev., 11, 3369-3389, 2018
https://doi.org/10.5194/gmd-11-3369-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Model description paper 21 Aug 2018

Model description paper | 21 Aug 2018

ORACLE 2-D (v2.0): an efficient module to compute the volatility and oxygen content of organic aerosol with a global chemistry–climate model

Alexandra P. Tsimpidi et al.
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Cited articles  
Ahmadov, R., McKeen, S. A., Robinson, A. L., Bahreini, R., Middlebrook, A. M., de Gouw, J. A., Meagher, J., Hsie, E. Y., Edgerton, E., Shaw, S., and Trainer, M.: A volatility basis set model for summertime secondary organic aerosols over the eastern United States in 2006, J. Geophys. Res.-Atmos., 117, D06301, https://doi.org/10.1029/2011jd016831, 2012. 
Allan, J. D., Williams, P. I., Morgan, W. T., Martin, C. L., Flynn, M. J., Lee, J., Nemitz, E., Phillips, G. J., Gallagher, M. W., and Coe, H.: Contributions from transport, solid fuel burning and cooking to primary organic aerosols in two UK cities, Atmos. Chem. Phys., 10, 647–668, https://doi.org/10.5194/acp-10-647-2010, 2010. 
Athanasopoulou, E., Vogel, H., Vogel, B., Tsimpidi, A. P., Pandis, S. N., Knote, C., and Fountoukis, C.: Modeling the meteorological and chemical effects of secondary organic aerosols during an EUCAARI campaign, Atmos. Chem. Phys., 13, 625–645, https://doi.org/10.5194/acp-13-625-2013, 2013. 
Bacer, S., Sullivan, S. C., Karydis, V. A., Barahona, D., Krämer, M., Nenes, A., Tost, H., Tsimpidi, A. P., Lelieveld, J., and Pozzer, A.: Implementation of a comprehensive ice crystal formation parameterization for cirrus and mixed-phase clouds into the EMAC model (based on MESSy 2.53), Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2018-62, in review, 2018. 
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A new module, ORACLE 2-D, that calculates the concentrations of surrogate organic species in two-dimensional space defined by volatility and oxygen-to-carbon ratio has been developed and evaluated. ORACLE 2-D uses a simple photochemical aging scheme that efficiently simulates the net effects of fragmentation and functionalization. ORACLE 2-D can be used to compute the ability of organic particles to act as cloud condensation nuclei and serves as a tool to quantify their climatic impact.
A new module, ORACLE 2-D, that calculates the concentrations of surrogate organic species in...
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