Articles | Volume 12, issue 7
https://doi.org/10.5194/gmd-12-2983-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/gmd-12-2983-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Development and technical paper
| 
15 Jul 2019
Development and technical paper |
| 15 Jul 2019
| 15 Jul 2019
A simplified parameterization of isoprene-epoxydiol-derived secondary organic aerosol (IEPOX-SOA) for global chemistry and climate models: a case study with GEOS-Chem v11-02-rc
Duseong S. Jo
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Alma Hodzic
Atmospheric Chemistry Observations and Modeling Lab., National Center for Atmospheric Research, Boulder, CO, USA
Laboratoire d'Aérologie, Université de Toulouse, CNRS, UPS,
Toulouse, France
Louisa K. Emmons
Atmospheric Chemistry Observations and Modeling Lab., National Center for Atmospheric Research, Boulder, CO, USA
Eloise A. Marais
Department of Physics and Astronomy, University of Leicester,
Leicester, UK
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Benjamin A. Nault
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Weiwei Hu
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Pedro Campuzano-Jost
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Jose L. Jimenez
CORRESPONDING AUTHOR
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
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22 citations as recorded by crossref.
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- Evaluation of Biogenic Organic Aerosols in the Amazon Rainforest Using WRF‐Chem With MOSAIC J. Mao et al. 10.1029/2021JD034913
- Isoprene Epoxydiol-Derived Sulfated and Nonsulfated Oligomers Suppress Particulate Mass Loss during Oxidative Aging of Secondary Organic Aerosol N. Armstrong et al. 10.1021/acs.est.2c03200
- Observationally Constrained Modeling of the Reactive Uptake of Isoprene-Derived Epoxydiols under Elevated Relative Humidity and Varying Acidity of Seed Aerosol Conditions J. Zhang et al. 10.1021/acsearthspacechem.2c00358
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- Climate Forcing and Trends of Organic Aerosols in the Community Earth System Model (CESM2) S. Tilmes et al. 10.1029/2019MS001827
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- Technical note: Improved synthetic routes to cis- and trans-(2-methyloxirane-2,3-diyl)dimethanol (cis- and trans-β-isoprene epoxydiol) M. Frauenheim et al. 10.5194/acp-23-7859-2023
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- Impacts of marine organic emissions on low-level stratiform clouds – a large eddy simulator study M. Prank et al. 10.5194/acp-22-10971-2022
- Exploring the Factors Controlling the Long‐Term Trend (1988–2019) of Surface Organic Aerosols in the Continental United States by Simulations Y. Liu et al. 10.1029/2022JD037935
- Biogenic volatile organic compounds in different ecosystems in Southern Kenya Y. Liu et al. 10.1016/j.atmosenv.2020.118064
22 citations as recorded by crossref.
- Exploration of oxidative chemistry and secondary organic aerosol formation in the Amazon during the wet season: explicit modeling of the Manaus urban plume with GECKO-A C. Mouchel-Vallon et al. 10.5194/acp-20-5995-2020
- PM2.5 Exposure and Associated Premature Mortality to 2100 in China Under Climate and Socioeconomic Change Scenarios B. Zou et al. 10.1029/2022EF003416
- Current State of Atmospheric Aerosol Thermodynamics and Mass Transfer Modeling: A Review K. Semeniuk & A. Dastoor 10.3390/atmos11020156
- Identifying chemical aerosol signatures using optical suborbital observations: how much can optical properties tell us about aerosol composition? M. Kacenelenbogen et al. 10.5194/acp-22-3713-2022
- Evaluation of Biogenic Organic Aerosols in the Amazon Rainforest Using WRF‐Chem With MOSAIC J. Mao et al. 10.1029/2021JD034913
- Isoprene Epoxydiol-Derived Sulfated and Nonsulfated Oligomers Suppress Particulate Mass Loss during Oxidative Aging of Secondary Organic Aerosol N. Armstrong et al. 10.1021/acs.est.2c03200
- Observationally Constrained Modeling of the Reactive Uptake of Isoprene-Derived Epoxydiols under Elevated Relative Humidity and Varying Acidity of Seed Aerosol Conditions J. Zhang et al. 10.1021/acsearthspacechem.2c00358
- Future changes in isoprene-epoxydiol-derived secondary organic aerosol (IEPOX SOA) under the Shared Socioeconomic Pathways: the importance of physicochemical dependency D. Jo et al. 10.5194/acp-21-3395-2021
- The C5–Alkene Triol Conundrum: Structural Characterization and Quantitation of Isoprene-Derived C5H10O3 Reactive Uptake Products M. Frauenheim et al. 10.1021/acs.estlett.2c00548
- Climate Forcing and Trends of Organic Aerosols in the Community Earth System Model (CESM2) S. Tilmes et al. 10.1029/2019MS001827
- An evaluation of global organic aerosol schemes using airborne observations S. Pai et al. 10.5194/acp-20-2637-2020
- Analysis of secondary organic aerosol simulation bias in the Community Earth System Model (CESM2.1) Y. Liu et al. 10.5194/acp-21-8003-2021
- A new simplified parameterization of secondary organic aerosol in the Community Earth System Model Version 2 (CESM2; CAM6.3) D. Jo et al. 10.5194/gmd-16-3893-2023
- Global–regional nested simulation of particle number concentration by combing microphysical processes with an evolving organic aerosol module X. Chen et al. 10.5194/acp-21-9343-2021
- Technical note: Improved synthetic routes to cis- and trans-(2-methyloxirane-2,3-diyl)dimethanol (cis- and trans-β-isoprene epoxydiol) M. Frauenheim et al. 10.5194/acp-23-7859-2023
- Long-term observational constraints of organic aerosol dependence on inorganic species in the southeast US Y. Zheng et al. 10.5194/acp-20-13091-2020
- Future air quality and premature mortality in Korea Y. Oak et al. 10.1016/j.scitotenv.2022.161134
- Uncertainties from biomass burning aerosols in air quality models obscure public health impacts in Southeast Asia M. Marvin et al. 10.5194/acp-24-3699-2024
- Aerosol pH indicator and organosulfate detectability from aerosol mass spectrometry measurements M. Schueneman et al. 10.5194/amt-14-2237-2021
- Impacts of marine organic emissions on low-level stratiform clouds – a large eddy simulator study M. Prank et al. 10.5194/acp-22-10971-2022
- Exploring the Factors Controlling the Long‐Term Trend (1988–2019) of Surface Organic Aerosols in the Continental United States by Simulations Y. Liu et al. 10.1029/2022JD037935
- Biogenic volatile organic compounds in different ecosystems in Southern Kenya Y. Liu et al. 10.1016/j.atmosenv.2020.118064
Latest update: 17 Apr 2024
Short summary
We developed a parameterization method for IEPOX-SOA based on the detailed chemical mechanism. Our parameterizations were tested using a box model and 3-D chemical transport model, which accurately captured the spatiotemporal distribution and response to changes in emissions compared to the explicit full chemistry, while being more computationally efficient. The method developed in this study can be applied to global climate models for long-term studies with a lower computational cost.
We developed a parameterization method for IEPOX-SOA based on the detailed chemical mechanism....
