Articles | Volume 7, issue 5
https://doi.org/10.5194/gmd-7-1855-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/gmd-7-1855-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Refinement of a model for evaluating the population exposure in an urban area
J. Soares
Finnish Meteorological Institute, Erik Palménin aukio 1, P.O. Box 503, 00101 Helsinki, Finland
A. Kousa
Helsinki Region Environmental Services Authority P.O. Box 521, 00521 Helsinki, Finland
J. Kukkonen
Finnish Meteorological Institute, Erik Palménin aukio 1, P.O. Box 503, 00101 Helsinki, Finland
L. Matilainen
Helsinki Region Environmental Services Authority P.O. Box 521, 00521 Helsinki, Finland
L. Kangas
Finnish Meteorological Institute, Erik Palménin aukio 1, P.O. Box 503, 00101 Helsinki, Finland
M. Kauhaniemi
Finnish Meteorological Institute, Erik Palménin aukio 1, P.O. Box 503, 00101 Helsinki, Finland
K. Riikonen
Finnish Meteorological Institute, Erik Palménin aukio 1, P.O. Box 503, 00101 Helsinki, Finland
J.-P. Jalkanen
Finnish Meteorological Institute, Erik Palménin aukio 1, P.O. Box 503, 00101 Helsinki, Finland
T. Rasila
Finnish Meteorological Institute, Erik Palménin aukio 1, P.O. Box 503, 00101 Helsinki, Finland
O. Hänninen
National Institute for Health and Welfare, P.O. Box 95, 70701 Kuopio, Finland
T. Koskentalo
Helsinki Region Environmental Services Authority P.O. Box 521, 00521 Helsinki, Finland
M. Aarnio
Finnish Meteorological Institute, Erik Palménin aukio 1, P.O. Box 503, 00101 Helsinki, Finland
C. Hendriks
TNO, department of Climate, Air and Sustainability, Utrecht, The Netherlands
A. Karppinen
Finnish Meteorological Institute, Erik Palménin aukio 1, P.O. Box 503, 00101 Helsinki, Finland
Related authors
Michael Boy, Erik S. Thomson, Juan-C. Acosta Navarro, Olafur Arnalds, Ekaterina Batchvarova, Jaana Bäck, Frank Berninger, Merete Bilde, Zoé Brasseur, Pavla Dagsson-Waldhauserova, Dimitri Castarède, Maryam Dalirian, Gerrit de Leeuw, Monika Dragosics, Ella-Maria Duplissy, Jonathan Duplissy, Annica M. L. Ekman, Keyan Fang, Jean-Charles Gallet, Marianne Glasius, Sven-Erik Gryning, Henrik Grythe, Hans-Christen Hansson, Margareta Hansson, Elisabeth Isaksson, Trond Iversen, Ingibjorg Jonsdottir, Ville Kasurinen, Alf Kirkevåg, Atte Korhola, Radovan Krejci, Jon Egill Kristjansson, Hanna K. Lappalainen, Antti Lauri, Matti Leppäranta, Heikki Lihavainen, Risto Makkonen, Andreas Massling, Outi Meinander, E. Douglas Nilsson, Haraldur Olafsson, Jan B. C. Pettersson, Nønne L. Prisle, Ilona Riipinen, Pontus Roldin, Meri Ruppel, Matthew Salter, Maria Sand, Øyvind Seland, Heikki Seppä, Henrik Skov, Joana Soares, Andreas Stohl, Johan Ström, Jonas Svensson, Erik Swietlicki, Ksenia Tabakova, Throstur Thorsteinsson, Aki Virkkula, Gesa A. Weyhenmeyer, Yusheng Wu, Paul Zieger, and Markku Kulmala
Atmos. Chem. Phys., 19, 2015–2061, https://doi.org/10.5194/acp-19-2015-2019, https://doi.org/10.5194/acp-19-2015-2019, 2019
Short summary
Short summary
The Nordic Centre of Excellence CRAICC (Cryosphere–Atmosphere Interactions in a Changing Arctic Climate), funded by NordForsk in the years 2011–2016, is the largest joint Nordic research and innovation initiative to date and aimed to strengthen research and innovation regarding climate change issues in the Nordic region. The paper presents an overview of the main scientific topics investigated and provides a state-of-the-art comprehensive summary of what has been achieved in CRAICC.
Joana Soares, Paul Andrew Makar, Yayne Aklilu, and Ayodeji Akingunola
Atmos. Chem. Phys., 18, 6543–6566, https://doi.org/10.5194/acp-18-6543-2018, https://doi.org/10.5194/acp-18-6543-2018, 2018
Short summary
Short summary
Grouping data on the basis of (dis)similarity can be used to assess the efficacy of monitoring networks. The data are cross-compared in terms of temporal variation and magnitude of concentrations, and sites are ranked according to their level of potential redundancy. The methodology can be applied to measurement data, helping to identify sites with different measuring technologies or data flaws, and to model output, generating maps of areas of spatial representativeness of a monitoring site.
Meri M. Ruppel, Joana Soares, Jean-Charles Gallet, Elisabeth Isaksson, Tõnu Martma, Jonas Svensson, Jack Kohler, Christina A. Pedersen, Sirkku Manninen, Atte Korhola, and Johan Ström
Atmos. Chem. Phys., 17, 12779–12795, https://doi.org/10.5194/acp-17-12779-2017, https://doi.org/10.5194/acp-17-12779-2017, 2017
Short summary
Short summary
Black carbon (BC) deposition enhances Arctic warming and melting. We present Svalbard ice core BC data from 2005 to 2015, comparing the results with chemical transport model data. The ice core and modelled BC deposition trends clearly deviate from measured and observed atmospheric concentration trends, and thus meteorological processes such as precipitation and scavenging efficiency seem to have a stronger influence on the BC deposition trend than BC emission or atmospheric concentration trends.
Joana Soares, Mikhail Sofiev, Camilla Geels, Jens H. Christensen, Camilla Andersson, Svetlana Tsyro, and Joakim Langner
Atmos. Chem. Phys., 16, 13081–13104, https://doi.org/10.5194/acp-16-13081-2016, https://doi.org/10.5194/acp-16-13081-2016, 2016
Short summary
Short summary
Multi-model comparison of four offline dispersion models driven by the global climate projection climate show that the major driver for the sea salt flux changes will be the seawater temperature, but there are substantial differences between the model predictions. The impact on regional radiative budget due to sea spray is considerable in the Mediterranean area, due to warmer temperatures and longer days during the winter.
M. Sofiev, J. Vira, R. Kouznetsov, M. Prank, J. Soares, and E. Genikhovich
Geosci. Model Dev., 8, 3497–3522, https://doi.org/10.5194/gmd-8-3497-2015, https://doi.org/10.5194/gmd-8-3497-2015, 2015
Short summary
Short summary
The paper presents a transport mechanism of SILAM CTM based on an algorithm of M. Galperin. We describe the original scheme and its updates needed for applications to long-living species, complex atmospheric flows, etc. The scheme is connected to vertical diffusion, chemical transformation and deposition algorithms. Quality of the advection routine is evaluated with a large set of tests, which showed performance fully comparable with state-of-the-art algorithms at much lower computational costs.
D. Simpson, C. Andersson, J.H. Christensen, M. Engardt, C. Geels, A. Nyiri, M. Posch, J. Soares, M. Sofiev, P. Wind, and J. Langner
Atmos. Chem. Phys., 14, 6995–7017, https://doi.org/10.5194/acp-14-6995-2014, https://doi.org/10.5194/acp-14-6995-2014, 2014
Heidi Hellén, Rostislav Kouznetsov, Kaisa Kraft, Jukka Seppälä, Mika Vestenius, Jukka-Pekka Jalkanen, Lauri Laakso, and Hannele Hakola
Atmos. Chem. Phys., 24, 4717–4731, https://doi.org/10.5194/acp-24-4717-2024, https://doi.org/10.5194/acp-24-4717-2024, 2024
Short summary
Short summary
Mixing ratios of C2-C5 NMHCs and methanethiol were measured on an island in the Baltic Sea using an in situ gas chromatograph. Shipping emissions were found to be an important source of ethene, ethyne, propene, and benzene. High summertime mixing ratios of methanethiol and dependence of mixing ratios on seawater temperature and height indicated the biogenic origin to possibly be phytoplankton or macroalgae. These emissions may have a strong impact on SO2 production and new particle formation.
Ville-Veikko Paunu, Niko Karvosenoja, David Segersson, Susana López-Aparicio, Ole-Kenneth Nielsen, Marlene Schmidt Plejdrup, Throstur Thorsteinsson, Dam Thanh Vo, Jeroen Kuenen, Hugo Denier van der Gon, Jukka-Pekka Jalkanen, Jørgen Brandt, and Camilla Geels
Earth Syst. Sci. Data, 16, 1453–1474, https://doi.org/10.5194/essd-16-1453-2024, https://doi.org/10.5194/essd-16-1453-2024, 2024
Short summary
Short summary
Air pollution is an important cause of adverse health effects, even in Nordic countries. To assess their health impacts, emission inventories with high spatial resolution are needed. We studied how national data and methods for the spatial distribution of the emissions compare to a European level inventory. For road transport the methods are well established, but for machinery and off-road emissions the current recommendations for the spatial distribution of these emissions should be improved.
Leena Kangas, Jaakko Kukkonen, Mari Kauhaniemi, Kari Riikonen, Mikhail Sofiev, Anu Kousa, Jarkko V. Niemi, and Ari Karppinen
Atmos. Chem. Phys., 24, 1489–1507, https://doi.org/10.5194/acp-24-1489-2024, https://doi.org/10.5194/acp-24-1489-2024, 2024
Short summary
Short summary
Residential wood combustion is a major source of fine particulate matter. This study has evaluated the contribution of residential wood combustion to fine particle concentrations and its year-to-year and seasonal variation in te Helsinki metropolitan area. The average concentrations attributed to wood combustion in winter were up to 10- or 15-fold compared to summer. Wood combustion caused 12 % to 14 % of annual fine particle concentrations. In winter, the contribution ranged from 16 % to 21 %.
Peter Manshausen, Duncan Watson-Parris, Matthew W. Christensen, Jukka-Pekka Jalkanen, and Philip Stier
Atmos. Chem. Phys., 23, 12545–12555, https://doi.org/10.5194/acp-23-12545-2023, https://doi.org/10.5194/acp-23-12545-2023, 2023
Short summary
Short summary
Aerosol from burning fuel changes cloud properties, e.g., the number of droplets and the content of water. Here, we study how clouds respond to different amounts of shipping aerosol. Droplet numbers increase linearly with increasing aerosol over a broad range until they stop increasing, while the amount of liquid water always increases, independently of emission amount. These changes in cloud properties can make them reflect more or less sunlight, which is important for the earth's climate.
Lea Fink, Matthias Karl, Volker Matthias, Sonia Oppo, Richard Kranenburg, Jeroen Kuenen, Sara Jutterström, Jana Moldanova, Elisa Majamäki, and Jukka-Pekka Jalkanen
Atmos. Chem. Phys., 23, 10163–10189, https://doi.org/10.5194/acp-23-10163-2023, https://doi.org/10.5194/acp-23-10163-2023, 2023
Short summary
Short summary
The Mediterranean Sea is a heavily trafficked shipping area, and air quality monitoring stations in numerous cities along the Mediterranean coast have detected high levels of air pollutants originating from shipping emissions. The current study investigates how existing restrictions on shipping-related emissions to the atmosphere ensure compliance with legislation. Focus was laid on fine particles and particle species, which were simulated with five different chemical transport models.
Antonin Soulie, Claire Granier, Sabine Darras, Nicolas Zilbermann, Thierno Doumbia, Marc Guevara, Jukka-Pekka Jalkanen, Sekou Keita, Cathy Liousse, Monica Crippa, Diego Guizzardi, Rachel Hoesly, and Steven Smith
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2023-306, https://doi.org/10.5194/essd-2023-306, 2023
Revised manuscript accepted for ESSD
Short summary
Short summary
Anthropogenic emissions are the result of transportation, power generation, industrial, residential and commercial activities, waste treatment and agriculture practices. This paper describes the new CAMS-GLOB-ANT gridded inventory of 2000–2023 anthropogenic emissions of air pollutants and greenhouse gases. The methodology to generate the emissions is explained, and the datasets are analysed and compared with publicly available global and regional inventories for selected world regions.
Sanna Saarikoski, Heidi Hellén, Arnaud P. Praplan, Simon Schallhart, Petri Clusius, Jarkko V. Niemi, Anu Kousa, Toni Tykkä, Rostislav Kouznetsov, Minna Aurela, Laura Salo, Topi Rönkkö, Luis M. F. Barreira, Liisa Pirjola, and Hilkka Timonen
Atmos. Chem. Phys., 23, 2963–2982, https://doi.org/10.5194/acp-23-2963-2023, https://doi.org/10.5194/acp-23-2963-2023, 2023
Short summary
Short summary
This study elucidates properties and sources of volatile organic compounds (VOCs) and organic aerosol (OA) in a traffic environment. Anthropogenic VOCs (aVOCs) were clearly higher than biogenic VOCs (bVOCs), but bVOCs produced a larger portion of oxidation products. OA consisted mostly of oxygenated OA, representing secondary OA (SOA). SOA was partly associated with bVOCs, but it was also related to long-range transport. Primary OA originated mostly from traffic.
Lea Fink, Matthias Karl, Volker Matthias, Sonia Oppo, Richard Kranenburg, Jeroen Kuenen, Jana Moldanova, Sara Jutterström, Jukka-Pekka Jalkanen, and Elisa Majamäki
Atmos. Chem. Phys., 23, 1825–1862, https://doi.org/10.5194/acp-23-1825-2023, https://doi.org/10.5194/acp-23-1825-2023, 2023
Short summary
Short summary
Potential ship impact on air pollution in the Mediterranean Sea was simulated with five chemistry transport models. An evaluation of the results for NO2 and O3 air concentrations and dry deposition is presented. Emission data, modeled year and domain were the same. Model run outputs were compared to measurements from background stations. We focused on comparing model outputs regarding the concentration of regulatory pollutants and the relative ship impact on total air pollution concentrations.
Svetlana Sofieva, Eija Asmi, Nina S. Atanasova, Aino E. Heikkinen, Emeline Vidal, Jonathan Duplissy, Martin Romantschuk, Rostislav Kouznetsov, Jaakko Kukkonen, Dennis H. Bamford, Antti-Pekka Hyvärinen, and Mikhail Sofiev
Atmos. Meas. Tech., 15, 6201–6219, https://doi.org/10.5194/amt-15-6201-2022, https://doi.org/10.5194/amt-15-6201-2022, 2022
Short summary
Short summary
A new bubble-generating glass chamber design with an extensive set of aerosol production experiments is presented to re-evaluate bubble-bursting-mediated aerosol production as a function of water parameters: bubbling air flow, water salinity, and temperature. Our main findings suggest modest dependence of aerosol production on the water salinity and a strong dependence on temperature below ~ 10 °C.
Marc Guevara, Hervé Petetin, Oriol Jorba, Hugo Denier van der Gon, Jeroen Kuenen, Ingrid Super, Jukka-Pekka Jalkanen, Elisa Majamäki, Lasse Johansson, Vincent-Henri Peuch, and Carlos Pérez García-Pando
Earth Syst. Sci. Data, 14, 2521–2552, https://doi.org/10.5194/essd-14-2521-2022, https://doi.org/10.5194/essd-14-2521-2022, 2022
Short summary
Short summary
To control the spread of the COVID-19 disease, European governments implemented mobility restriction measures that resulted in an unprecedented drop in anthropogenic emissions. This work presents a dataset of emission adjustment factors that allows quantifying changes in 2020 European primary emissions per country and pollutant sector at the daily scale. The resulting dataset can be used as input in modelling studies aiming at quantifying the impact of COVID-19 on air quality levels.
Jaakko Kukkonen, Juha Nikmo, Kari Riikonen, Ilmo Westerholm, Pekko Ilvessalo, Tuomo Bergman, and Klaus Haikarainen
Geosci. Model Dev., 15, 4027–4054, https://doi.org/10.5194/gmd-15-4027-2022, https://doi.org/10.5194/gmd-15-4027-2022, 2022
Short summary
Short summary
A mathematical model has been developed for the dispersion of plumes originating from major fires. We have refined the model for the early evolution of the fire plumes; such a module has not been previously presented. We have evaluated the model against experimental field-scale data. The predicted concentrations agreed well with the aircraft measurements. We have also compiled an operational version of the model, which can be used for emergency contingency planning in the case of major fires.
Matthias Karl, Liisa Pirjola, Tiia Grönholm, Mona Kurppa, Srinivasan Anand, Xiaole Zhang, Andreas Held, Rolf Sander, Miikka Dal Maso, David Topping, Shuai Jiang, Leena Kangas, and Jaakko Kukkonen
Geosci. Model Dev., 15, 3969–4026, https://doi.org/10.5194/gmd-15-3969-2022, https://doi.org/10.5194/gmd-15-3969-2022, 2022
Short summary
Short summary
The community aerosol dynamics model MAFOR includes several advanced features: coupling with an up-to-date chemistry mechanism for volatile organic compounds, a revised Brownian coagulation kernel that takes into account the fractal geometry of soot particles, a multitude of nucleation parameterizations, size-resolved partitioning of semi-volatile inorganics, and a hybrid method for the formation of secondary organic aerosols within the framework of condensation and evaporation.
Joel Kuula, Hilkka Timonen, Jarkko V. Niemi, Hanna E. Manninen, Topi Rönkkö, Tareq Hussein, Pak Lun Fung, Sasu Tarkoma, Mikko Laakso, Erkka Saukko, Aino Ovaska, Markku Kulmala, Ari Karppinen, Lasse Johansson, and Tuukka Petäjä
Atmos. Chem. Phys., 22, 4801–4808, https://doi.org/10.5194/acp-22-4801-2022, https://doi.org/10.5194/acp-22-4801-2022, 2022
Short summary
Short summary
Modern and up-to-date policies and air quality management strategies are instrumental in tackling global air pollution. As the European Union is preparing to revise Ambient Air Quality Directive 2008/50/EC, this paper initiates discussion on selected features of the directive that we believe would benefit from a reassessment. The scientific community has the most recent and deepest understanding of air pollution; thus, its contribution is essential.
Ranjeet S. Sokhi, Nicolas Moussiopoulos, Alexander Baklanov, John Bartzis, Isabelle Coll, Sandro Finardi, Rainer Friedrich, Camilla Geels, Tiia Grönholm, Tomas Halenka, Matthias Ketzel, Androniki Maragkidou, Volker Matthias, Jana Moldanova, Leonidas Ntziachristos, Klaus Schäfer, Peter Suppan, George Tsegas, Greg Carmichael, Vicente Franco, Steve Hanna, Jukka-Pekka Jalkanen, Guus J. M. Velders, and Jaakko Kukkonen
Atmos. Chem. Phys., 22, 4615–4703, https://doi.org/10.5194/acp-22-4615-2022, https://doi.org/10.5194/acp-22-4615-2022, 2022
Short summary
Short summary
This review of air quality research focuses on developments over the past decade. The article considers current and future challenges that are important from air quality research and policy perspectives and highlights emerging prominent gaps of knowledge. The review also examines how air pollution management needs to adapt to new challenges and makes recommendations to guide the direction for future air quality research within the wider community and to provide support for policy.
Pak Lun Fung, Martha A. Zaidan, Jarkko V. Niemi, Erkka Saukko, Hilkka Timonen, Anu Kousa, Joel Kuula, Topi Rönkkö, Ari Karppinen, Sasu Tarkoma, Markku Kulmala, Tuukka Petäjä, and Tareq Hussein
Atmos. Chem. Phys., 22, 1861–1882, https://doi.org/10.5194/acp-22-1861-2022, https://doi.org/10.5194/acp-22-1861-2022, 2022
Short summary
Short summary
We developed an input-adaptive mixed-effects model, which was automatised to select the best combination of input variables, including up to three fixed effect variables and three time indictors as random effect variables. We tested the model to estimate lung-deposited surface area (LDSA), which correlates well with human health. The results show the inclusion of time indicators improved the sensitivity and the accuracy of the model so that it could serve as a network of virtual sensors.
Jeroen Kuenen, Stijn Dellaert, Antoon Visschedijk, Jukka-Pekka Jalkanen, Ingrid Super, and Hugo Denier van der Gon
Earth Syst. Sci. Data, 14, 491–515, https://doi.org/10.5194/essd-14-491-2022, https://doi.org/10.5194/essd-14-491-2022, 2022
Short summary
Short summary
This paper presents an 18-year time series for anthropogenic emissions for the main air pollutants in Europe, distinguishing 15 main source categories. It provides a complete overview of emissions to air and is designed to support air quality modelling. The data build where possible on official country total emissions used in the policy processes, but where necessary alternative data were used. The emission data are spatially distributed at high resolution (~ 6 km x 6 km) in a consistent way.
Marcus Reckermann, Anders Omstedt, Tarmo Soomere, Juris Aigars, Naveed Akhtar, Magdalena Bełdowska, Jacek Bełdowski, Tom Cronin, Michał Czub, Margit Eero, Kari Petri Hyytiäinen, Jukka-Pekka Jalkanen, Anders Kiessling, Erik Kjellström, Karol Kuliński, Xiaoli Guo Larsén, Michelle McCrackin, H. E. Markus Meier, Sonja Oberbeckmann, Kevin Parnell, Cristian Pons-Seres de Brauwer, Anneli Poska, Jarkko Saarinen, Beata Szymczycha, Emma Undeman, Anders Wörman, and Eduardo Zorita
Earth Syst. Dynam., 13, 1–80, https://doi.org/10.5194/esd-13-1-2022, https://doi.org/10.5194/esd-13-1-2022, 2022
Short summary
Short summary
As part of the Baltic Earth Assessment Reports (BEAR), we present an inventory and discussion of different human-induced factors and processes affecting the environment of the Baltic Sea region and their interrelations. Some are naturally occurring and modified by human activities, others are completely human-induced, and they are all interrelated to different degrees. The findings from this study can largely be transferred to other comparable marginal and coastal seas in the world.
Jari Walden, Liisa Pirjola, Tuomas Laurila, Juha Hatakka, Heidi Pettersson, Tuomas Walden, Jukka-Pekka Jalkanen, Harri Nordlund, Toivo Truuts, Miika Meretoja, and Kimmo K. Kahma
Atmos. Chem. Phys., 21, 18175–18194, https://doi.org/10.5194/acp-21-18175-2021, https://doi.org/10.5194/acp-21-18175-2021, 2021
Short summary
Short summary
Ship emissions play an important role in the deposition of gaseous compounds and nanoparticles (Ntot), affecting climate, human health (especially in coastal areas), and eutrophication. Micrometeorological methods showed that ship emissions were mainly responsible for the deposition of Ntot, whereas they only accounted for a minor proportion of CO2 deposition. An uncertainty analysis applied to the fluxes and fuel sulfur content results demonstrated the reliability of the results.
Sanna Saarikoski, Jarkko V. Niemi, Minna Aurela, Liisa Pirjola, Anu Kousa, Topi Rönkkö, and Hilkka Timonen
Atmos. Chem. Phys., 21, 14851–14869, https://doi.org/10.5194/acp-21-14851-2021, https://doi.org/10.5194/acp-21-14851-2021, 2021
Short summary
Short summary
This study presents the main sources of black carbon (BC) at two urban environments. The largest fraction of BC originated from biomass burning at the residential site (38 %) and from vehicular emissions (57 %) in the street canyon. Also, a significant fraction of BC was associated with urban background or long-range transport. The data are needed by modelers and authorities when assessing climate and air quality impact of BC as well as directing the emission legislation and mitigation actions.
Camilla Geels, Morten Winther, Camilla Andersson, Jukka-Pekka Jalkanen, Jørgen Brandt, Lise M. Frohn, Ulas Im, Wing Leung, and Jesper H. Christensen
Atmos. Chem. Phys., 21, 12495–12519, https://doi.org/10.5194/acp-21-12495-2021, https://doi.org/10.5194/acp-21-12495-2021, 2021
Short summary
Short summary
In this study, we set up new shipping emissions scenarios and use two chemistry transport models and a health assessment model to assess the development of air quality and related health impacts in the Nordic region. Shipping alone is associated with about 850 premature deaths during present-day conditions, decreasing to approximately 550–600 cases in the 2050 scenarios.
Jukka-Pekka Jalkanen, Lasse Johansson, Magda Wilewska-Bien, Lena Granhag, Erik Ytreberg, K. Martin Eriksson, Daniel Yngsell, Ida-Maja Hassellöv, Kerstin Magnusson, Urmas Raudsepp, Ilja Maljutenko, Hulda Winnes, and Jana Moldanova
Ocean Sci., 17, 699–728, https://doi.org/10.5194/os-17-699-2021, https://doi.org/10.5194/os-17-699-2021, 2021
Short summary
Short summary
This modelling study describes a methodology for describing pollutant discharges from ships to the sea. The pilot area used is the Baltic Sea area and discharges of bilge, ballast, sewage, wash water as well as stern tube oil are reported for the year 2012. This work also reports the release of SOx scrubber effluents. This technique may be used by ships to comply with tight sulfur limits inside Emission Control Areas, but it also introduces a new pollutant stream from ships to the sea.
Luis M. F. Barreira, Aku Helin, Minna Aurela, Kimmo Teinilä, Milla Friman, Leena Kangas, Jarkko V. Niemi, Harri Portin, Anu Kousa, Liisa Pirjola, Topi Rönkkö, Sanna Saarikoski, and Hilkka Timonen
Atmos. Chem. Phys., 21, 6297–6314, https://doi.org/10.5194/acp-21-6297-2021, https://doi.org/10.5194/acp-21-6297-2021, 2021
Short summary
Short summary
We present results from the long-term measurements (5 years) of highly time-resolved atmospheric PM1 composition at an urban street canyon site. Overall, the results increased knowledge of the variability of PM1 concentration, composition, and sources in a traffic site and the implications for urban air quality. The investigation of pollution episodes showed that both local and long-range-transported pollutants can still cause elevated PM1 and PM2.5 concentrations in northern Europe.
Sami D. Seppälä, Joel Kuula, Antti-Pekka Hyvärinen, Sanna Saarikoski, Topi Rönkkö, Jorma Keskinen, Jukka-Pekka Jalkanen, and Hilkka Timonen
Atmos. Chem. Phys., 21, 3215–3234, https://doi.org/10.5194/acp-21-3215-2021, https://doi.org/10.5194/acp-21-3215-2021, 2021
Short summary
Short summary
The effects of fuel sulfur content restrictions implemented by the International Maritime Organization in the Baltic Sea (in July 2010 and January 2015) on the particle properties of ship exhaust plumes and ambient aerosol were studied. The restrictions reduced the particle number concentrations and median particle size in plumes and number concentrations in ambient aerosol. These changes may improve human health in coastal areas and decrease the cooling effect of exhaust emissions from ships.
Krista Luoma, Jarkko V. Niemi, Minna Aurela, Pak Lun Fung, Aku Helin, Tareq Hussein, Leena Kangas, Anu Kousa, Topi Rönkkö, Hilkka Timonen, Aki Virkkula, and Tuukka Petäjä
Atmos. Chem. Phys., 21, 1173–1189, https://doi.org/10.5194/acp-21-1173-2021, https://doi.org/10.5194/acp-21-1173-2021, 2021
Short summary
Short summary
This study combined black carbon measurements from 15 Finnish sites that represented different environments (traffic, detached housing area, urban background, and regional background). The seasonal and diurnal variations in the black carbon concentration were associated with local emissions from traffic and residential wood burning. The study observed decreasing trends in the black carbon concentration and associated them with decreases in traffic emissions.
Jan Eiof Jonson, Michael Gauss, Michael Schulz, Jukka-Pekka Jalkanen, and Hilde Fagerli
Atmos. Chem. Phys., 20, 11399–11422, https://doi.org/10.5194/acp-20-11399-2020, https://doi.org/10.5194/acp-20-11399-2020, 2020
Short summary
Short summary
We have calculated the effects of air pollution in Europe from shipping on levels of PM2.5 and ozone and depositions of oxidised nitrogen and sulfur from individual sea areas and from all global shipping. Model results are shown for Europe as a whole but also focusing on select, mainly coastal, countries. Calculations are made using 2017 emissions supplemented by calculations reducing sulfur emissions from ships by about 80 % following the implementation of the 2020 global sulfur cap.
Lasse Johansson, Erik Ytreberg, Jukka-Pekka Jalkanen, Erik Fridell, K. Martin Eriksson, Maria Lagerström, Ilja Maljutenko, Urmas Raudsepp, Vivian Fischer, and Eva Roth
Ocean Sci., 16, 1143–1163, https://doi.org/10.5194/os-16-1143-2020, https://doi.org/10.5194/os-16-1143-2020, 2020
Short summary
Short summary
Very little is currently known about the activities and emissions of private leisure boats. To change this, a new model was created (BEAM). The model was used for the Baltic Sea to estimate leisure boat emissions, also considering antifouling paint leach. When compared to commercial shipping, the modeled leisure boat emissions were seen to be surprisingly large for some pollutant species, and these emissions were heavily concentrated on coastal inhabited areas during summer and early autumn.
Rafael A. O. Nunes, Maria C. M. Alvim-Ferraz, Fernando G. Martins, Fátima Calderay-Cayetano, Vanessa Durán-Grados, Juan Moreno-Gutiérrez, Jukka-Pekka Jalkanen, Hanna Hannuniemi, and Sofia I. V. Sousa
Atmos. Chem. Phys., 20, 9473–9489, https://doi.org/10.5194/acp-20-9473-2020, https://doi.org/10.5194/acp-20-9473-2020, 2020
Short summary
Short summary
The central position of the Iberian Peninsula with ship traffic between the Americas, Africa, and Europe, combined with the known adverse effects of this sector on air quality, emphasises the relevance of a more detailed study of these impacts in this region. Results showed increased levels of SO2 and NO2 near port areas, as well as of O3, sulfate, PM2.5, and PM10 over the Iberian Peninsula coastline due to shipping emissions. To study mitigation measures, application is crucial.
Jaakko Kukkonen, Mikko Savolahti, Yuliia Palamarchuk, Timo Lanki, Väinö Nurmi, Ville-Veikko Paunu, Leena Kangas, Mikhail Sofiev, Ari Karppinen, Androniki Maragkidou, Pekka Tiittanen, and Niko Karvosenoja
Atmos. Chem. Phys., 20, 9371–9391, https://doi.org/10.5194/acp-20-9371-2020, https://doi.org/10.5194/acp-20-9371-2020, 2020
Short summary
Short summary
We have developed a mathematical model that can be used to analyse the benefits that could be achieved by implementing alternative air quality abatement measures, policies or strategies. The model was applied to determine pollution sources in the whole of Finland in 2015. Clearly the most economically effective measures were the reduction in emissions from low-level sources in urban areas. Such sources include road transport, non-road vehicles and machinery, and residential wood combustion.
Lin Tang, Martin O. P. Ramacher, Jana Moldanová, Volker Matthias, Matthias Karl, Lasse Johansson, Jukka-Pekka Jalkanen, Katarina Yaramenka, Armin Aulinger, and Malin Gustafsson
Atmos. Chem. Phys., 20, 7509–7530, https://doi.org/10.5194/acp-20-7509-2020, https://doi.org/10.5194/acp-20-7509-2020, 2020
Short summary
Short summary
The effects of shipping emissions on air quality and health in the harbour city of Gothenburg were simulated for 2012 with coupled regional and city-scale chemistry transport models. The results show that contributions of shipping to exposure and health impacts from particulate matter and NO2 are significant and that shipping-related exposure to PM is dominated by emissions from regional shipping outside the city domain and is larger than exposure related to emissions from local road traffic.
Jaakko Kukkonen, Susana López-Aparicio, David Segersson, Camilla Geels, Leena Kangas, Mari Kauhaniemi, Androniki Maragkidou, Anne Jensen, Timo Assmuth, Ari Karppinen, Mikhail Sofiev, Heidi Hellén, Kari Riikonen, Juha Nikmo, Anu Kousa, Jarkko V. Niemi, Niko Karvosenoja, Gabriela Sousa Santos, Ingrid Sundvor, Ulas Im, Jesper H. Christensen, Ole-Kenneth Nielsen, Marlene S. Plejdrup, Jacob Klenø Nøjgaard, Gunnar Omstedt, Camilla Andersson, Bertil Forsberg, and Jørgen Brandt
Atmos. Chem. Phys., 20, 4333–4365, https://doi.org/10.5194/acp-20-4333-2020, https://doi.org/10.5194/acp-20-4333-2020, 2020
Short summary
Short summary
Residential wood combustion can cause substantial emissions of fine particulate matter and adverse health effects. This study has, for the first time, evaluated the impacts of residential wood combustion in a harmonised manner in four Nordic cities. Wood combustion caused major shares of fine particle concentrations in Oslo (up to 60 %) and Umeå (up to 30 %) and also notable shares in Copenhagen (up to 20 %) and Helsinki (up to 15 %).
Jan Eiof Jonson, Michael Gauss, Jukka-Pekka Jalkanen, and Lasse Johansson
Atmos. Chem. Phys., 19, 13469–13487, https://doi.org/10.5194/acp-19-13469-2019, https://doi.org/10.5194/acp-19-13469-2019, 2019
Short summary
Short summary
Calculations have been made with the regional-scale EMEP chemical transport model covering Europe and the sea areas surrounding Europe, including much of the North Atlantic. The main focus is on the effects on air pollution as well as depositions of sulfur and nitrogen following the implementation of stricter sulfur emission regulations from 1 January 2015 for ships operating in the Baltic Sea. We also include a study on the effects of future (2030) emissions changes.
Ulas Im, Jesper H. Christensen, Ole-Kenneth Nielsen, Maria Sand, Risto Makkonen, Camilla Geels, Camilla Anderson, Jaakko Kukkonen, Susana Lopez-Aparicio, and Jørgen Brandt
Atmos. Chem. Phys., 19, 12975–12992, https://doi.org/10.5194/acp-19-12975-2019, https://doi.org/10.5194/acp-19-12975-2019, 2019
Short summary
Short summary
Sectoral contributions of anthropogenic emissions in Denmark, Finland, Norway and Sweden on air pollution and mortality over the Nordic and the Arctic regions are calculated. 80 % of PM2.5 over the Nordic countries is transported from outside Scandinavia. Residential combustion, industry and traffic are the main sectors to be targeted in emission mitigation. Exposure to ambient air pollution in the Nordic countries leads to more than 10 000 deaths in the region annually and costs EUR 7 billion.
Ana Stojiljkovic, Mari Kauhaniemi, Jaakko Kukkonen, Kaarle Kupiainen, Ari Karppinen, Bruce Rolstad Denby, Anu Kousa, Jarkko V. Niemi, and Matthias Ketzel
Atmos. Chem. Phys., 19, 11199–11212, https://doi.org/10.5194/acp-19-11199-2019, https://doi.org/10.5194/acp-19-11199-2019, 2019
Short summary
Short summary
Nordic countries experience the deterioration of air quality in springtime due to high PM10 concentrations. Non-exhaust emissions from vehicular traffic are regarded as the most significant source of particulate air pollution during this time of year. The results from this study demonstrate the fact that changes in winter tyre types and adjustments to road maintenance could substantially reduce non-exhaust emissions.
Martin Otto Paul Ramacher, Matthias Karl, Johannes Bieser, Jukka-Pekka Jalkanen, and Lasse Johansson
Atmos. Chem. Phys., 19, 9153–9179, https://doi.org/10.5194/acp-19-9153-2019, https://doi.org/10.5194/acp-19-9153-2019, 2019
Short summary
Short summary
We simulated the impact of NOx shipping emissions on air quality and exposure in the Baltic Sea harbour cities Rostock (Germany), Riga (Latvia) and Gdańsk–Gdynia (Poland) for 2012. We found that local shipping affects total NO2, with contributions of 22 %, 11 % and 16 % in Rostock, Riga and Gdańsk–Gdynia. Exposure to NO2 from all emission sources was highest at home addresses (54 %–59 %). Emissions from shipping have a high impact on NO2 exposure in the port area (50 %–80 %).
Matthias Karl, Jan Eiof Jonson, Andreas Uppstu, Armin Aulinger, Marje Prank, Mikhail Sofiev, Jukka-Pekka Jalkanen, Lasse Johansson, Markus Quante, and Volker Matthias
Atmos. Chem. Phys., 19, 7019–7053, https://doi.org/10.5194/acp-19-7019-2019, https://doi.org/10.5194/acp-19-7019-2019, 2019
Short summary
Short summary
The effect of ship emissions on the regional air quality in the Baltic Sea region was investigated with three regional chemistry transport model systems. The ship influence on air quality is shown to depend on the boundary conditions, meteorological data and aerosol formation and deposition schemes that are used in these models. The study provides a reliable approach for the evaluation of policy options regarding emission regulations for ship traffic in the Baltic Sea.
Michael Boy, Erik S. Thomson, Juan-C. Acosta Navarro, Olafur Arnalds, Ekaterina Batchvarova, Jaana Bäck, Frank Berninger, Merete Bilde, Zoé Brasseur, Pavla Dagsson-Waldhauserova, Dimitri Castarède, Maryam Dalirian, Gerrit de Leeuw, Monika Dragosics, Ella-Maria Duplissy, Jonathan Duplissy, Annica M. L. Ekman, Keyan Fang, Jean-Charles Gallet, Marianne Glasius, Sven-Erik Gryning, Henrik Grythe, Hans-Christen Hansson, Margareta Hansson, Elisabeth Isaksson, Trond Iversen, Ingibjorg Jonsdottir, Ville Kasurinen, Alf Kirkevåg, Atte Korhola, Radovan Krejci, Jon Egill Kristjansson, Hanna K. Lappalainen, Antti Lauri, Matti Leppäranta, Heikki Lihavainen, Risto Makkonen, Andreas Massling, Outi Meinander, E. Douglas Nilsson, Haraldur Olafsson, Jan B. C. Pettersson, Nønne L. Prisle, Ilona Riipinen, Pontus Roldin, Meri Ruppel, Matthew Salter, Maria Sand, Øyvind Seland, Heikki Seppä, Henrik Skov, Joana Soares, Andreas Stohl, Johan Ström, Jonas Svensson, Erik Swietlicki, Ksenia Tabakova, Throstur Thorsteinsson, Aki Virkkula, Gesa A. Weyhenmeyer, Yusheng Wu, Paul Zieger, and Markku Kulmala
Atmos. Chem. Phys., 19, 2015–2061, https://doi.org/10.5194/acp-19-2015-2019, https://doi.org/10.5194/acp-19-2015-2019, 2019
Short summary
Short summary
The Nordic Centre of Excellence CRAICC (Cryosphere–Atmosphere Interactions in a Changing Arctic Climate), funded by NordForsk in the years 2011–2016, is the largest joint Nordic research and innovation initiative to date and aimed to strengthen research and innovation regarding climate change issues in the Nordic region. The paper presents an overview of the main scientific topics investigated and provides a state-of-the-art comprehensive summary of what has been achieved in CRAICC.
Matthias Karl, Johannes Bieser, Beate Geyer, Volker Matthias, Jukka-Pekka Jalkanen, Lasse Johansson, and Erik Fridell
Atmos. Chem. Phys., 19, 1721–1752, https://doi.org/10.5194/acp-19-1721-2019, https://doi.org/10.5194/acp-19-1721-2019, 2019
Short summary
Short summary
Air emissions of nitrogen oxides from ship traffic in the Baltic Sea are a health concern in coastal areas of the Baltic Sea region. We find that the introduction of the nitrogen emission control area (NECA) is critical for reducing ship emissions of nitrogen oxides to levels that are low enough to sustainably dampen ozone production. The decline of the ship-related nitrogen deposition to the Baltic Sea between 2012 and 2040 varies between 46 % and 78 % in different regulation scenarios.
Jukka-Pekka Jalkanen, Lasse Johansson, Mattias Liefvendahl, Rickard Bensow, Peter Sigray, Martin Östberg, Ilkka Karasalo, Mathias Andersson, Heikki Peltonen, and Jukka Pajala
Ocean Sci., 14, 1373–1383, https://doi.org/10.5194/os-14-1373-2018, https://doi.org/10.5194/os-14-1373-2018, 2018
Short summary
Short summary
This paper presents the implementation of an underwater noise emission module in the Ship Traffic Emission Assessment Model. This model is based on real shipping activity, as described by the vessel navigation systems, and combines it with technical descriptions of each ship. The methodology described facilitates the expression of underwater noise as emission maps, which describe the energy emitted to the water. This enables regular reporting of shipping noise and facilitates further research.
Leena Järvi, Üllar Rannik, Tom V. Kokkonen, Mona Kurppa, Ari Karppinen, Rostislav D. Kouznetsov, Pekka Rantala, Timo Vesala, and Curtis R. Wood
Atmos. Meas. Tech., 11, 5421–5438, https://doi.org/10.5194/amt-11-5421-2018, https://doi.org/10.5194/amt-11-5421-2018, 2018
Short summary
Short summary
Identical EC systems on two sides of a building in central Helsinki were used to assess the uncertainty of the vertical fluxes on the single measurement point from July 2013 to September 2015. Sampling at only one point yielded up to 12% underestimation in the cumulative carbon fluxes; for sensible and latent heat the respective values were up to 5 and 8%. The commonly used statistics, kurtosis and skewness, are not necessarily suitable for filtering out data in a densely built urban area.
Jaakko Kukkonen, Leena Kangas, Mari Kauhaniemi, Mikhail Sofiev, Mia Aarnio, Jouni J. K. Jaakkola, Anu Kousa, and Ari Karppinen
Atmos. Chem. Phys., 18, 8041–8064, https://doi.org/10.5194/acp-18-8041-2018, https://doi.org/10.5194/acp-18-8041-2018, 2018
Short summary
Short summary
We have quantified the emissions and concentrations of fine particulate matter in the Helsinki area for an unprecedentedly extensive period, from 1980 to 2014. The modelled concentrations agree well with the measured data. The concentrations of fine particles have decreased drastically since the 1980s, to about a half of the highest values. The results make it possible to evaluate the long-term health impacts of air pollution substantially better.
Joana Soares, Paul Andrew Makar, Yayne Aklilu, and Ayodeji Akingunola
Atmos. Chem. Phys., 18, 6543–6566, https://doi.org/10.5194/acp-18-6543-2018, https://doi.org/10.5194/acp-18-6543-2018, 2018
Short summary
Short summary
Grouping data on the basis of (dis)similarity can be used to assess the efficacy of monitoring networks. The data are cross-compared in terms of temporal variation and magnitude of concentrations, and sites are ranked according to their level of potential redundancy. The methodology can be applied to measurement data, helping to identify sites with different measuring technologies or data flaws, and to model output, generating maps of areas of spatial representativeness of a monitoring site.
Martijn Schaap, Sabine Banzhaf, Thomas Scheuschner, Markus Geupel, Carlijn Hendriks, Richard Kranenburg, Hans-Dieter Nagel, Arjo J. Segers, Angela von Schlutow, Roy Wichink Kruit, and Peter J. H. Builtjes
Biogeosciences Discuss., https://doi.org/10.5194/bg-2017-491, https://doi.org/10.5194/bg-2017-491, 2017
Revised manuscript has not been submitted
Short summary
Short summary
Deposition of nitrogen and sulfur from the atmosphere on ecosystems causes a loss of biodiversity. We used a combination of atmospheric modelling and deposition observations to estimate the deposition to ecosystems across Germany. We estimate that 70 % of the ecosystems in Germany receive too much nitrogen from deposition. The results are used to determine whether economic activities causing nitrogen emissions are allowed in sensitive areas.
Astrid M. M. Manders, Peter J. H. Builtjes, Lyana Curier, Hugo A. C. Denier van der Gon, Carlijn Hendriks, Sander Jonkers, Richard Kranenburg, Jeroen J. P. Kuenen, Arjo J. Segers, Renske M. A. Timmermans, Antoon J. H. Visschedijk, Roy J. Wichink Kruit, W. Addo J. van Pul, Ferd J. Sauter, Eric van der Swaluw, Daan P. J. Swart, John Douros, Henk Eskes, Erik van Meijgaard, Bert van Ulft, Peter van Velthoven, Sabine Banzhaf, Andrea C. Mues, Rainer Stern, Guangliang Fu, Sha Lu, Arnold Heemink, Nils van Velzen, and Martijn Schaap
Geosci. Model Dev., 10, 4145–4173, https://doi.org/10.5194/gmd-10-4145-2017, https://doi.org/10.5194/gmd-10-4145-2017, 2017
Short summary
Short summary
The regional-scale air quality model LOTOS–EUROS has been developed by a consortium of Dutch institutes. Recently, version 2.0 of the model was released as an open-source version. Next to a technical description and model evaluation for 2012, this paper presents the model developments in context of the history of air quality modelling and provides an outlook for future directions. Key and innovative applications of LOTOS–EUROS are also highlighted.
Meri M. Ruppel, Joana Soares, Jean-Charles Gallet, Elisabeth Isaksson, Tõnu Martma, Jonas Svensson, Jack Kohler, Christina A. Pedersen, Sirkku Manninen, Atte Korhola, and Johan Ström
Atmos. Chem. Phys., 17, 12779–12795, https://doi.org/10.5194/acp-17-12779-2017, https://doi.org/10.5194/acp-17-12779-2017, 2017
Short summary
Short summary
Black carbon (BC) deposition enhances Arctic warming and melting. We present Svalbard ice core BC data from 2005 to 2015, comparing the results with chemical transport model data. The ice core and modelled BC deposition trends clearly deviate from measured and observed atmospheric concentration trends, and thus meteorological processes such as precipitation and scavenging efficiency seem to have a stronger influence on the BC deposition trend than BC emission or atmospheric concentration trends.
John Backman, Curtis R. Wood, Mikko Auvinen, Leena Kangas, Hanna Hannuniemi, Ari Karppinen, and Jaakko Kukkonen
Geosci. Model Dev., 10, 3793–3803, https://doi.org/10.5194/gmd-10-3793-2017, https://doi.org/10.5194/gmd-10-3793-2017, 2017
Short summary
Short summary
Meteorological input parameters for urban- and local-scale dispersion models can be derived from meteorological observations. This study presents a sensitivity analysis of a meteorological model that utilises readily available meteorological data to derive specific parameters required to model the atmospheric dispersion of pollutants. The study shows that wind speed is the most fundamental meteorological input parameter followed by solar radiation.
Heidi Hellén, Leena Kangas, Anu Kousa, Mika Vestenius, Kimmo Teinilä, Ari Karppinen, Jaakko Kukkonen, and Jarkko V. Niemi
Atmos. Chem. Phys., 17, 3475–3487, https://doi.org/10.5194/acp-17-3475-2017, https://doi.org/10.5194/acp-17-3475-2017, 2017
Short summary
Short summary
Estimating impacts of wood combustion on ambient levels of PAHs is challenging. In this study effect of residential wood combustion on the benzo[a]pyrene concentrations in the air of Helsinki metropolitan area was studied, using ambient air measurements, emission estimates and dispersion modeling. Combining all this information enabled a quantitative characterization of the influence of residential wood combustion, which was found to be the main local source and more important than for PM2.5.
Joana Soares, Mikhail Sofiev, Camilla Geels, Jens H. Christensen, Camilla Andersson, Svetlana Tsyro, and Joakim Langner
Atmos. Chem. Phys., 16, 13081–13104, https://doi.org/10.5194/acp-16-13081-2016, https://doi.org/10.5194/acp-16-13081-2016, 2016
Short summary
Short summary
Multi-model comparison of four offline dispersion models driven by the global climate projection climate show that the major driver for the sea salt flux changes will be the seawater temperature, but there are substantial differences between the model predictions. The impact on regional radiative budget due to sea spray is considerable in the Mediterranean area, due to warmer temperatures and longer days during the winter.
Marje Prank, Mikhail Sofiev, Svetlana Tsyro, Carlijn Hendriks, Valiyaveetil Semeena, Xavier Vazhappilly Francis, Tim Butler, Hugo Denier van der Gon, Rainer Friedrich, Johannes Hendricks, Xin Kong, Mark Lawrence, Mattia Righi, Zissis Samaras, Robert Sausen, Jaakko Kukkonen, and Ranjeet Sokhi
Atmos. Chem. Phys., 16, 6041–6070, https://doi.org/10.5194/acp-16-6041-2016, https://doi.org/10.5194/acp-16-6041-2016, 2016
Short summary
Short summary
Aerosol composition in Europe was simulated by four chemistry transport models and compared to observations to identify the most prominent areas for model improvement. Notable differences were found between the models' predictions, attributable to different treatment or omission of aerosol sources and processes. All models underestimated the observed concentrations by 10–60 %, mostly due to under-predicting the carbonaceous and mineral particles and omitting the aerosol-bound water.
Joonas Enroth, Sanna Saarikoski, Jarkko Niemi, Anu Kousa, Irena Ježek, Griša Močnik, Samara Carbone, Heino Kuuluvainen, Topi Rönkkö, Risto Hillamo, and Liisa Pirjola
Atmos. Chem. Phys., 16, 5497–5512, https://doi.org/10.5194/acp-16-5497-2016, https://doi.org/10.5194/acp-16-5497-2016, 2016
Short summary
Short summary
This paper presents a comprehensive summary of roadside measurements using a mobile laboratory, equipped with state-of-the-art instrumentation. Pollution gradients were observed for particle number, black carbon, organics, some metals, and gases at four different highway environments. Flow dynamics appeared to be an important factor, however, at the most open site, condensation of semi-volatile organics was observed. The fleet average NO2 emission factor increased over the last decade.
Matthias Karl, Jaakko Kukkonen, Menno P. Keuken, Susanne Lützenkirchen, Liisa Pirjola, and Tareq Hussein
Atmos. Chem. Phys., 16, 4817–4835, https://doi.org/10.5194/acp-16-4817-2016, https://doi.org/10.5194/acp-16-4817-2016, 2016
Short summary
Short summary
Particles emitted from road traffic are subject to complex dilution processes as well as microphysical transformation processes. Particle measurements at major roads in Rotterdam, Oslo and Helsinki were used to analyze the relevance of microphysical transformation processes. Transformation processes caused changes of the particle number concentration of up to 20–30 % on the neighborhood scale. A simple parameterization to predict particle number concentrations in urban areas is presented.
Louis Marelle, Jennie L. Thomas, Jean-Christophe Raut, Kathy S. Law, Jukka-Pekka Jalkanen, Lasse Johansson, Anke Roiger, Hans Schlager, Jin Kim, Anja Reiter, and Bernadett Weinzierl
Atmos. Chem. Phys., 16, 2359–2379, https://doi.org/10.5194/acp-16-2359-2016, https://doi.org/10.5194/acp-16-2359-2016, 2016
J. Kukkonen, M. Karl, M. P. Keuken, H. A. C. Denier van der Gon, B. R. Denby, V. Singh, J. Douros, A. Manders, Z. Samaras, N. Moussiopoulos, S. Jonkers, M. Aarnio, A. Karppinen, L. Kangas, S. Lützenkirchen, T. Petäjä, I. Vouitsis, and R. S. Sokhi
Geosci. Model Dev., 9, 451–478, https://doi.org/10.5194/gmd-9-451-2016, https://doi.org/10.5194/gmd-9-451-2016, 2016
Short summary
Short summary
For analyzing the health effects of particulate matter, it is necessary to consider not only the mass of particles, but also their sizes and composition. A simple measure for the former is the number concentration of particles. We present particle number concentrations in five major European cities, namely Helsinki, Oslo, London, Rotterdam, and Athens, in 2008, based mainly on modelling. The concentrations of PN were mostly influenced by the emissions from local vehicular traffic.
J.-P. Jalkanen, L. Johansson, and J. Kukkonen
Atmos. Chem. Phys., 16, 71–84, https://doi.org/10.5194/acp-16-71-2016, https://doi.org/10.5194/acp-16-71-2016, 2016
Short summary
Short summary
This manuscript describes the emissions from shipping in European sea areas. The work is based on automatic position reports (AIS) sent by ships and reflects realistic activity patterns of ships. The work demonstrates that it is feasible to construct full bottom-up emission inventories based on large-volume activity data sets.
M. Sofiev, J. Vira, R. Kouznetsov, M. Prank, J. Soares, and E. Genikhovich
Geosci. Model Dev., 8, 3497–3522, https://doi.org/10.5194/gmd-8-3497-2015, https://doi.org/10.5194/gmd-8-3497-2015, 2015
Short summary
Short summary
The paper presents a transport mechanism of SILAM CTM based on an algorithm of M. Galperin. We describe the original scheme and its updates needed for applications to long-living species, complex atmospheric flows, etc. The scheme is connected to vertical diffusion, chemical transformation and deposition algorithms. Quality of the advection routine is evaluated with a large set of tests, which showed performance fully comparable with state-of-the-art algorithms at much lower computational costs.
J. Beecken, J. Mellqvist, K. Salo, J. Ekholm, J.-P. Jalkanen, L. Johansson, V. Litvinenko, K. Volodin, and D. A. Frank-Kamenetsky
Atmos. Chem. Phys., 15, 5229–5241, https://doi.org/10.5194/acp-15-5229-2015, https://doi.org/10.5194/acp-15-5229-2015, 2015
Short summary
Short summary
Measurements of SO2, NOx and particle emission factors of more than 400 individual ship passages in the Gulf of Finland are presented and discussed. The measurements were conducted during two campaigns in the years 2011 and 2012 from ground-based and helicopter-based platforms. It was found that a significant number of ships use fuel oil with a fuel sulfur content below the limit of 1%.
Additionally, the results of modeled data for the same ships were compared to the measurements of this study.
J. E. Jonson, J. P. Jalkanen, L. Johansson, M. Gauss, and H. A. C. Denier van der Gon
Atmos. Chem. Phys., 15, 783–798, https://doi.org/10.5194/acp-15-783-2015, https://doi.org/10.5194/acp-15-783-2015, 2015
Short summary
Short summary
In order to assess the effects of ship emissions in and around the
Baltic Sea and the North Sea, regional model calculations are made
with the EMEP air pollution model. Ship emissions are based on
accurate ship positioning data. The effects on depositions and air
pollution and the resulting number of years of life lost (YOLLs)
are calculated by comparing model calculations with and without
ship emissions, with ship emissions before and after 2010, and for future
projections.
J. Kukkonen, J. Nikmo, M. Sofiev, K. Riikonen, T. Petäjä, A. Virkkula, J. Levula, S. Schobesberger, and D. M. Webber
Geosci. Model Dev., 7, 2663–2681, https://doi.org/10.5194/gmd-7-2663-2014, https://doi.org/10.5194/gmd-7-2663-2014, 2014
M. Kauhaniemi, A. Stojiljkovic, L. Pirjola, A. Karppinen, J. Härkönen, K. Kupiainen, L. Kangas, M. A. Aarnio, G. Omstedt, B. R. Denby, and J. Kukkonen
Atmos. Chem. Phys., 14, 9155–9169, https://doi.org/10.5194/acp-14-9155-2014, https://doi.org/10.5194/acp-14-9155-2014, 2014
J. M. Balzani Lööv, B. Alfoldy, L. F. L. Gast, J. Hjorth, F. Lagler, J. Mellqvist, J. Beecken, N. Berg, J. Duyzer, H. Westrate, D. P. J. Swart, A. J. C. Berkhout, J.-P. Jalkanen, A. J. Prata, G. R. van der Hoff, and A. Borowiak
Atmos. Meas. Tech., 7, 2597–2613, https://doi.org/10.5194/amt-7-2597-2014, https://doi.org/10.5194/amt-7-2597-2014, 2014
I. Ialongo, J. Hakkarainen, N. Hyttinen, J.-P. Jalkanen, L. Johansson, K. F. Boersma, N. Krotkov, and J. Tamminen
Atmos. Chem. Phys., 14, 7795–7805, https://doi.org/10.5194/acp-14-7795-2014, https://doi.org/10.5194/acp-14-7795-2014, 2014
D. Simpson, C. Andersson, J.H. Christensen, M. Engardt, C. Geels, A. Nyiri, M. Posch, J. Soares, M. Sofiev, P. Wind, and J. Langner
Atmos. Chem. Phys., 14, 6995–7017, https://doi.org/10.5194/acp-14-6995-2014, https://doi.org/10.5194/acp-14-6995-2014, 2014
J. Beecken, J. Mellqvist, K. Salo, J. Ekholm, and J.-P. Jalkanen
Atmos. Meas. Tech., 7, 1957–1968, https://doi.org/10.5194/amt-7-1957-2014, https://doi.org/10.5194/amt-7-1957-2014, 2014
A. Virkkula, J. Levula, T. Pohja, P. P. Aalto, P. Keronen, S. Schobesberger, C. B. Clements, L. Pirjola, A.-J. Kieloaho, L. Kulmala, H. Aaltonen, J. Patokoski, J. Pumpanen, J. Rinne, T. Ruuskanen, M. Pihlatie, H. E. Manninen, V. Aaltonen, H. Junninen, T. Petäjä, J. Backman, M. Dal Maso, T. Nieminen, T. Olsson, T. Grönholm, J. Aalto, T. H. Virtanen, M. Kajos, V.-M. Kerminen, D. M. Schultz, J. Kukkonen, M. Sofiev, G. De Leeuw, J. Bäck, P. Hari, and M. Kulmala
Atmos. Chem. Phys., 14, 4473–4502, https://doi.org/10.5194/acp-14-4473-2014, https://doi.org/10.5194/acp-14-4473-2014, 2014
A. Mues, J. Kuenen, C. Hendriks, A. Manders, A. Segers, Y. Scholz, C. Hueglin, P. Builtjes, and M. Schaap
Atmos. Chem. Phys., 14, 939–955, https://doi.org/10.5194/acp-14-939-2014, https://doi.org/10.5194/acp-14-939-2014, 2014
L. Pirjola, A. Pajunoja, J. Walden, J.-P. Jalkanen, T. Rönkkö, A. Kousa, and T. Koskentalo
Atmos. Meas. Tech., 7, 149–161, https://doi.org/10.5194/amt-7-149-2014, https://doi.org/10.5194/amt-7-149-2014, 2014
L. Johansson, J.-P. Jalkanen, J. Kalli, and J. Kukkonen
Atmos. Chem. Phys., 13, 11375–11389, https://doi.org/10.5194/acp-13-11375-2013, https://doi.org/10.5194/acp-13-11375-2013, 2013
R. Kranenburg, A. J. Segers, C. Hendriks, and M. Schaap
Geosci. Model Dev., 6, 721–733, https://doi.org/10.5194/gmd-6-721-2013, https://doi.org/10.5194/gmd-6-721-2013, 2013
Related subject area
Atmospheric sciences
Modelling wind farm effects in HARMONIE–AROME (cycle 43.2.2) – Part 1: Implementation and evaluation
Analytical and adaptable initial conditions for dry and moist baroclinic waves in the global hydrostatic model OpenIFS (CY43R3)
Challenges of constructing and selecting the “perfect” boundary conditions for the large-eddy simulation model PALM
A machine learning approach for evaluating Southern Ocean cloud radiative biases in a global atmosphere model
Decision Support System version 1.0 (DSS v1.0) for air quality management in Delhi, India
How non-equilibrium aerosol chemistry impacts particle acidity: the GMXe AERosol CHEMistry (GMXe–AERCHEM, v1.0) sub-submodel of MESSy
A grid model for vertical correction of precipitable water vapor over the Chinese mainland and surrounding areas using random forest
MEXPLORER 1.0.0 – a mechanism explorer for analysis and visualization of chemical reaction pathways based on graph theory
Advances and prospects of deep learning for medium-range extreme weather forecasting
An overview of the Western United States Dynamically Downscaled Dataset (WUS-D3)
cloudbandPy 1.0: an automated algorithm for the detection of tropical–extratropical cloud bands
PyRTlib: an educational Python-based library for non-scattering atmospheric microwave radiative transfer computations
Deep learning applied to CO2 power plant emissions quantification using simulated satellite images
Sensitivity of the WRF-Chem v4.4 simulations of ozone and formaldehyde and their precursors to multiple bottom-up emission inventories over East Asia during the KORUS-AQ 2016 field campaign
Optimising urban measurement networks for CO2 flux estimation: a high-resolution observing system simulation experiment using GRAMM/GRAL
Assessment of climate biases in OpenIFS version 43r3 across model horizontal resolutions and time steps
High-resolution multi-scaling of outdoor human thermal comfort and its intra-urban variability based on machine learning
Effects of vertical grid spacing on the climate simulated in the ICON-Sapphire global storm-resolving model
Development of the tangent linear and adjoint models of the global online chemical transport model MPAS-CO2 v7.3
Impacts of updated reaction kinetics on the global GEOS-Chem simulation of atmospheric chemistry
Spatial spin-up of precipitation in limited-area convection-permitting simulations over North America using the CRCM6/GEM5.0 model
Sensitivity of atmospheric rivers to aerosol treatment in regional climate simulations: insights from the AIRA identification algorithm
The implementation of dust mineralogy in COSMO5.05-MUSCAT
Implementation of the ISORROPIA-lite aerosol thermodynamics model into the EMAC chemistry climate model (based on MESSy v2.55): implications for aerosol composition and acidity
Evaluation of surface shortwave downward radiation forecasts by the numerical weather prediction model AROME
GEO4PALM v1.1: an open-source geospatial data processing toolkit for the PALM model system
Modeling collision–coalescence in particle microphysics: numerical convergence of mean and variance of precipitation in cloud simulations using the University of Warsaw Lagrangian Cloud Model (UWLCM) 2.1
Modeling below-cloud scavenging of size-resolved particles in GEM-MACHv3.1
Impacts of a double-moment bulk cloud microphysics scheme (NDW6-G23) on aerosol fields in NICAM.19 with a global 14 km grid resolution
Sensitivity of air quality model responses to emission changes: comparison of results based on four EU inventories through FAIRMODE benchmarking methodology
A simple and realistic aerosol emission approach for use in the Thompson–Eidhammer microphysics scheme in the NOAA UFS Weather Model (version GSL global-24Feb2022)
On the formation of biogenic secondary organic aerosol in chemical transport models: an evaluation of the WRF-CHIMERE (v2020r2) model with a focus over the Finnish boreal forest
The first application of a numerically exact, higher-order sensitivity analysis approach for atmospheric modelling: implementation of the hyperdual-step method in the Community Multiscale Air Quality Model (CMAQ) version 5.3.2
The ddeq Python library for point source quantification from remote sensing images (Version 1.0)
GAN-argcPredNet v2.0: a radar echo extrapolation model based on spatiotemporal process enhancement
Analysis of the GEFS-Aerosols annual budget to better understand aerosol predictions simulated in the model
A model for rapid PM2.5 exposure estimates in wildfire conditions using routinely available data: rapidfire v0.1.3
BoundaryLayerDynamics.jl v1.0: a modern codebase for atmospheric boundary-layer simulations
Investigating Ground-Level Ozone Pollution in Semi-Arid and Arid Regions of Arizona Using WRF-Chem v4.4 Modeling
The wave-age-dependent stress parameterisation (WASP) for momentum and heat turbulent fluxes at sea in SURFEX v8.1
FUME 2.0 – Flexible Universal processor for Modeling Emissions
Assessment of tropospheric ozone products from downscaled CAMS reanalysis and CAMS daily forecast using urban air quality monitoring stations in Iran
Application of regional meteorology and air quality models based on MIPS CPU Platform
Spherical air mass factors in one and two dimensions with SASKTRAN 1.6.0
An improved version of the piecewise parabolic method advection scheme: description and performance assessment in a bidimensional test case with stiff chemistry in toyCTM v1.0.1
INCHEM-Py v1.2: a community box model for indoor air chemistry
Implementation and evaluation of updated photolysis rates in the EMEP MSC-W chemistry-transport model using Cloud-J v7.3e
Representation of atmosphere-induced heterogeneity in land–atmosphere interactions in E3SM–MMFv2
How the meteorological spectral nudging impacts on aerosol radiation clouds interactions?
A General Comprehensive Evaluation Method for Cross-Scale Precipitation Forecasts
Jana Fischereit, Henrik Vedel, Xiaoli Guo Larsén, Natalie E. Theeuwes, Gregor Giebel, and Eigil Kaas
Geosci. Model Dev., 17, 2855–2875, https://doi.org/10.5194/gmd-17-2855-2024, https://doi.org/10.5194/gmd-17-2855-2024, 2024
Short summary
Short summary
Wind farms impact local wind and turbulence. To incorporate these effects in weather forecasting, the explicit wake parameterization (EWP) is added to the forecasting model HARMONIE–AROME. We evaluate EWP using flight data above and downstream of wind farms, comparing it with an alternative wind farm parameterization and another weather model. Results affirm the correct implementation of EWP, emphasizing the necessity of accounting for wind farm effects in accurate weather forecasting.
Clément Bouvier, Daan van den Broek, Madeleine Ekblom, and Victoria A. Sinclair
Geosci. Model Dev., 17, 2961–2986, https://doi.org/10.5194/gmd-17-2961-2024, https://doi.org/10.5194/gmd-17-2961-2024, 2024
Short summary
Short summary
An analytical initial background state has been developed for moist baroclinic wave simulation on an aquaplanet and implemented into OpenIFS. Seven parameters can be controlled, which are used to generate the background states and the development of baroclinic waves. The meteorological and numerical stability has been assessed. Resulting baroclinic waves have proven to be realistic and sensitive to the jet's width.
Jelena Radović, Michal Belda, Jaroslav Resler, Kryštof Eben, Martin Bureš, Jan Geletič, Pavel Krč, Hynek Řezníček, and Vladimír Fuka
Geosci. Model Dev., 17, 2901–2927, https://doi.org/10.5194/gmd-17-2901-2024, https://doi.org/10.5194/gmd-17-2901-2024, 2024
Short summary
Short summary
Boundary conditions are of crucial importance for numerical model (e.g., PALM) validation studies and have a large influence on the model results, especially when studying the atmosphere of real, complex, and densely built urban environments. Our experiments with different driving conditions for the large-eddy simulation model PALM show its strong dependency on boundary conditions, which is important for the proper separation of errors coming from the boundary conditions and the model itself.
Sonya L. Fiddes, Marc D. Mallet, Alain Protat, Matthew T. Woodhouse, Simon P. Alexander, and Kalli Furtado
Geosci. Model Dev., 17, 2641–2662, https://doi.org/10.5194/gmd-17-2641-2024, https://doi.org/10.5194/gmd-17-2641-2024, 2024
Short summary
Short summary
In this study we present an evaluation that considers complex, non-linear systems in a holistic manner. This study uses XGBoost, a machine learning algorithm, to predict the simulated Southern Ocean shortwave radiation bias in the ACCESS model using cloud property biases as predictors. We then used a novel feature importance analysis to quantify the role that each cloud bias plays in predicting the radiative bias, laying the foundation for advanced Earth system model evaluation and development.
Gaurav Govardhan, Sachin D. Ghude, Rajesh Kumar, Sumit Sharma, Preeti Gunwani, Chinmay Jena, Prafull Yadav, Shubhangi Ingle, Sreyashi Debnath, Pooja Pawar, Prodip Acharja, Rajmal Jat, Gayatry Kalita, Rupal Ambulkar, Santosh Kulkarni, Akshara Kaginalkar, Vijay K. Soni, Ravi S. Nanjundiah, and Madhavan Rajeevan
Geosci. Model Dev., 17, 2617–2640, https://doi.org/10.5194/gmd-17-2617-2024, https://doi.org/10.5194/gmd-17-2617-2024, 2024
Short summary
Short summary
A newly developed air quality forecasting framework, Decision Support System (DSS), for air quality management in Delhi, India, provides source attribution with numerous emission reduction scenarios besides forecasts. DSS shows that during post-monsoon and winter seasons, Delhi and its neighboring districts contribute to 30 %–40 % each to pollution in Delhi. On average, a 40 % reduction in the emissions in Delhi and the surrounding districts would result in a 24 % reduction in Delhi's pollution.
Simon Rosanka, Holger Tost, Rolf Sander, Patrick Jöckel, Astrid Kerkweg, and Domenico Taraborrelli
Geosci. Model Dev., 17, 2597–2615, https://doi.org/10.5194/gmd-17-2597-2024, https://doi.org/10.5194/gmd-17-2597-2024, 2024
Short summary
Short summary
The capabilities of the Modular Earth Submodel System (MESSy) are extended to account for non-equilibrium aqueous-phase chemistry in the representation of deliquescent aerosols. When applying the new development in a global simulation, we find that MESSy's bias in modelling routinely observed reduced inorganic aerosol mass concentrations, especially in the United States. Furthermore, the representation of fine-aerosol pH is particularly improved in the marine boundary layer.
Junyu Li, Yuxin Wang, Lilong Liu, Yibin Yao, Liangke Huang, and Feijuan Li
Geosci. Model Dev., 17, 2569–2581, https://doi.org/10.5194/gmd-17-2569-2024, https://doi.org/10.5194/gmd-17-2569-2024, 2024
Short summary
Short summary
In this study, we have developed a model (RF-PWV) to characterize precipitable water vapor (PWV) variation with altitude in the study area. RF-PWV can significantly reduce errors in vertical correction, enhance PWV fusion product accuracy, and provide insights into PWV vertical distribution, thereby contributing to climate research.
Rolf Sander
Geosci. Model Dev., 17, 2419–2425, https://doi.org/10.5194/gmd-17-2419-2024, https://doi.org/10.5194/gmd-17-2419-2024, 2024
Short summary
Short summary
The open-source software MEXPLORER 1.0.0 is presented here. The program can be used to analyze, reduce, and visualize complex chemical reaction mechanisms. The mathematics behind the tool is based on graph theory: chemical species are represented as vertices, and reactions as edges. MEXPLORER is a community model published under the GNU General Public License.
Leonardo Olivetti and Gabriele Messori
Geosci. Model Dev., 17, 2347–2358, https://doi.org/10.5194/gmd-17-2347-2024, https://doi.org/10.5194/gmd-17-2347-2024, 2024
Short summary
Short summary
In the last decades, weather forecasting up to 15 d into the future has been dominated by physics-based numerical models. Recently, deep learning models have challenged this paradigm. However, the latter models may struggle when forecasting weather extremes. In this article, we argue for deep learning models specifically designed to handle extreme events, and we propose a foundational framework to develop such models.
Stefan Rahimi, Lei Huang, Jesse Norris, Alex Hall, Naomi Goldenson, Will Krantz, Benjamin Bass, Chad Thackeray, Henry Lin, Di Chen, Eli Dennis, Ethan Collins, Zachary J. Lebo, Emily Slinskey, Sara Graves, Surabhi Biyani, Bowen Wang, Stephen Cropper, and the UCLA Center for Climate Science Team
Geosci. Model Dev., 17, 2265–2286, https://doi.org/10.5194/gmd-17-2265-2024, https://doi.org/10.5194/gmd-17-2265-2024, 2024
Short summary
Short summary
Here, we project future climate across the western United States through the end of the 21st century using a regional climate model, embedded within 16 latest-generation global climate models, to provide the community with a high-resolution physically based ensemble of climate data for use at local scales. Strengths and weaknesses of the data are frankly discussed as we overview the downscaled dataset.
Romain Pilon and Daniela I. V. Domeisen
Geosci. Model Dev., 17, 2247–2264, https://doi.org/10.5194/gmd-17-2247-2024, https://doi.org/10.5194/gmd-17-2247-2024, 2024
Short summary
Short summary
This paper introduces a new method for detecting atmospheric cloud bands to identify long convective cloud bands that extend from the tropics to the midlatitudes. The algorithm allows for easy use and enables researchers to study the life cycle and climatology of cloud bands and associated rainfall. This method provides insights into the large-scale processes involved in cloud band formation and their connections between different regions, as well as differences across ocean basins.
Salvatore Larosa, Domenico Cimini, Donatello Gallucci, Saverio Teodosio Nilo, and Filomena Romano
Geosci. Model Dev., 17, 2053–2076, https://doi.org/10.5194/gmd-17-2053-2024, https://doi.org/10.5194/gmd-17-2053-2024, 2024
Short summary
Short summary
PyRTlib is an attractive educational tool because it provides a flexible and user-friendly way to broadly simulate how electromagnetic radiation travels through the atmosphere as it interacts with atmospheric constituents (such as gases, aerosols, and hydrometeors). PyRTlib is a so-called radiative transfer model; these are commonly used to simulate and understand remote sensing observations from ground-based, airborne, or satellite instruments.
Joffrey Dumont Le Brazidec, Pierre Vanderbecken, Alban Farchi, Grégoire Broquet, Gerrit Kuhlmann, and Marc Bocquet
Geosci. Model Dev., 17, 1995–2014, https://doi.org/10.5194/gmd-17-1995-2024, https://doi.org/10.5194/gmd-17-1995-2024, 2024
Short summary
Short summary
Our research presents an innovative approach to estimating power plant CO2 emissions from satellite images of the corresponding plumes such as those from the forthcoming CO2M satellite constellation. The exploitation of these images is challenging due to noise and meteorological uncertainties. To overcome these obstacles, we use a deep learning neural network trained on simulated CO2 images. Our method outperforms alternatives, providing a positive perspective for the analysis of CO2M images.
Kyoung-Min Kim, Si-Wan Kim, Seunghwan Seo, Donald R. Blake, Seogju Cho, James H. Crawford, Louisa K. Emmons, Alan Fried, Jay R. Herman, Jinkyu Hong, Jinsang Jung, Gabriele G. Pfister, Andrew J. Weinheimer, Jung-Hun Woo, and Qiang Zhang
Geosci. Model Dev., 17, 1931–1955, https://doi.org/10.5194/gmd-17-1931-2024, https://doi.org/10.5194/gmd-17-1931-2024, 2024
Short summary
Short summary
Three emission inventories were evaluated for East Asia using data acquired during a field campaign in 2016. The inventories successfully reproduced the daily variations of ozone and nitrogen dioxide. However, the spatial distributions of model ozone did not fully agree with the observations. Additionally, all simulations underestimated carbon monoxide and volatile organic compound (VOC) levels. Increasing VOC emissions over South Korea resulted in improved ozone simulations.
Sanam Noreen Vardag and Robert Maiwald
Geosci. Model Dev., 17, 1885–1902, https://doi.org/10.5194/gmd-17-1885-2024, https://doi.org/10.5194/gmd-17-1885-2024, 2024
Short summary
Short summary
We use the atmospheric transport model GRAMM/GRAL in a Bayesian inversion to estimate urban CO2 emissions on a neighbourhood scale. We analyse the effect of varying number, precision and location of CO2 sensors for CO2 flux estimation. We further test the inclusion of co-emitted species and correlation in the inversion. The study showcases the general usefulness of GRAMM/GRAL in measurement network design.
Abhishek Savita, Joakim Kjellsson, Robin Pilch Kedzierski, Mojib Latif, Tabea Rahm, Sebastian Wahl, and Wonsun Park
Geosci. Model Dev., 17, 1813–1829, https://doi.org/10.5194/gmd-17-1813-2024, https://doi.org/10.5194/gmd-17-1813-2024, 2024
Short summary
Short summary
The OpenIFS model is used to examine the impact of horizontal resolutions (HR) and model time steps. We find that the surface wind biases over the oceans, in particular the Southern Ocean, are sensitive to the model time step and HR, with the HR having the smallest biases. When using a coarse-resolution model with a shorter time step, a similar improvement is also found. Climate biases can be reduced in the OpenIFS model at a cheaper cost by reducing the time step rather than increasing the HR.
Ferdinand Briegel, Jonas Wehrle, Dirk Schindler, and Andreas Christen
Geosci. Model Dev., 17, 1667–1688, https://doi.org/10.5194/gmd-17-1667-2024, https://doi.org/10.5194/gmd-17-1667-2024, 2024
Short summary
Short summary
We present a new approach to model heat stress in cities using artificial intelligence (AI). We show that the AI model is fast in terms of prediction but accurate when evaluated with measurements. The fast-predictive AI model enables several new potential applications, including heat stress prediction and warning; downscaling of potential future climates; evaluation of adaptation effectiveness; and, more fundamentally, development of guidelines to support urban planning and policymaking.
Hauke Schmidt, Sebastian Rast, Jiawei Bao, Amrit Cassim, Shih-Wei Fang, Diego Jimenez-de la Cuesta, Paul Keil, Lukas Kluft, Clarissa Kroll, Theresa Lang, Ulrike Niemeier, Andrea Schneidereit, Andrew I. L. Williams, and Bjorn Stevens
Geosci. Model Dev., 17, 1563–1584, https://doi.org/10.5194/gmd-17-1563-2024, https://doi.org/10.5194/gmd-17-1563-2024, 2024
Short summary
Short summary
A recent development in numerical simulations of the global atmosphere is the increase in horizontal resolution to grid spacings of a few kilometers. However, the vertical grid spacing of these models has not been reduced at the same rate as the horizontal grid spacing. Here, we assess the effects of much finer vertical grid spacings, in particular the impacts on cloud quantities and the atmospheric energy balance.
Tao Zheng, Sha Feng, Jeffrey Steward, Xiaoxu Tian, David Baker, and Martin Baxter
Geosci. Model Dev., 17, 1543–1562, https://doi.org/10.5194/gmd-17-1543-2024, https://doi.org/10.5194/gmd-17-1543-2024, 2024
Short summary
Short summary
The tangent linear and adjoint models have been successfully implemented in the MPAS-CO2 system, which has undergone rigorous accuracy testing. This development lays the groundwork for a global carbon flux data assimilation system, which offers the flexibility of high-resolution focus on specific areas, while maintaining a coarser resolution elsewhere. This approach significantly reduces computational costs and is thus perfectly suited for future CO2 geostationery and imager satellites.
Kelvin H. Bates, Mathew J. Evans, Barron H. Henderson, and Daniel J. Jacob
Geosci. Model Dev., 17, 1511–1524, https://doi.org/10.5194/gmd-17-1511-2024, https://doi.org/10.5194/gmd-17-1511-2024, 2024
Short summary
Short summary
Accurate representation of rates and products of chemical reactions in atmospheric models is crucial for simulating concentrations of pollutants and climate forcers. We update the widely used GEOS-Chem atmospheric chemistry model with reaction parameters from recent compilations of experimental data and demonstrate the implications for key atmospheric chemical species. The updates decrease tropospheric CO mixing ratios and increase stratospheric nitrogen oxide mixing ratios, among other changes.
François Roberge, Alejandro Di Luca, René Laprise, Philippe Lucas-Picher, and Julie Thériault
Geosci. Model Dev., 17, 1497–1510, https://doi.org/10.5194/gmd-17-1497-2024, https://doi.org/10.5194/gmd-17-1497-2024, 2024
Short summary
Short summary
Our study addresses a challenge in dynamical downscaling using regional climate models, focusing on the lack of small-scale features near the boundaries. We introduce a method to identify this “spatial spin-up” in precipitation simulations. Results show spin-up distances up to 300 km, varying by season and driving variable. Double nesting with comprehensive variables (e.g. microphysical variables) offers advantages. Findings will help optimize simulations for better climate projections.
Eloisa Raluy-López, Juan Pedro Montávez, and Pedro Jiménez-Guerrero
Geosci. Model Dev., 17, 1469–1495, https://doi.org/10.5194/gmd-17-1469-2024, https://doi.org/10.5194/gmd-17-1469-2024, 2024
Short summary
Short summary
Atmospheric rivers (ARs) represent a significant source of water but are also related to extreme precipitation events. Here, we present a new regional-scale AR identification algorithm and apply it to three simulations that include aerosol interactions at different levels. The results show that aerosols modify the intensity and trajectory of ARs and redistribute the AR-related precipitation. Thus, the correct inclusion of aerosol effects is important in the simulation of AR behavior.
Sofía Gómez Maqueo Anaya, Dietrich Althausen, Matthias Faust, Holger Baars, Bernd Heinold, Julian Hofer, Ina Tegen, Albert Ansmann, Ronny Engelmann, Annett Skupin, Birgit Heese, and Kerstin Schepanski
Geosci. Model Dev., 17, 1271–1295, https://doi.org/10.5194/gmd-17-1271-2024, https://doi.org/10.5194/gmd-17-1271-2024, 2024
Short summary
Short summary
Mineral dust aerosol particles vary greatly in their composition depending on source region, which leads to different physicochemical properties. Most atmosphere–aerosol models consider mineral dust aerosols to be compositionally homogeneous, which ultimately increases model uncertainty. Here, we present an approach to explicitly consider the heterogeneity of the mineralogical composition for simulations of the Saharan atmospheric dust cycle with regard to dust transport towards the Atlantic.
Alexandros Milousis, Alexandra P. Tsimpidi, Holger Tost, Spyros N. Pandis, Athanasios Nenes, Astrid Kiendler-Scharr, and Vlassis A. Karydis
Geosci. Model Dev., 17, 1111–1131, https://doi.org/10.5194/gmd-17-1111-2024, https://doi.org/10.5194/gmd-17-1111-2024, 2024
Short summary
Short summary
This study aims to evaluate the newly developed ISORROPIA-lite aerosol thermodynamic module within the EMAC model and explore discrepancies in global atmospheric simulations of aerosol composition and acidity by utilizing different aerosol phase states. Even though local differences were found in regions where the RH ranged from 20 % to 60 %, on a global scale the results are similar. Therefore, ISORROPIA-lite can be a reliable and computationally effective alternative to ISORROPIA II in EMAC.
Marie-Adèle Magnaldo, Quentin Libois, Sébastien Riette, and Christine Lac
Geosci. Model Dev., 17, 1091–1109, https://doi.org/10.5194/gmd-17-1091-2024, https://doi.org/10.5194/gmd-17-1091-2024, 2024
Short summary
Short summary
With the worldwide development of the solar energy sector, the need for reliable solar radiation forecasts has significantly increased. However, meteorological models that predict, among others things, solar radiation have errors. Therefore, we wanted to know in which situtaions these errors are most significant. We found that errors mostly occur in cloudy situations, and different errors were highlighted depending on the cloud altitude. Several potential sources of errors were identified.
Dongqi Lin, Jiawei Zhang, Basit Khan, Marwan Katurji, and Laura E. Revell
Geosci. Model Dev., 17, 815–845, https://doi.org/10.5194/gmd-17-815-2024, https://doi.org/10.5194/gmd-17-815-2024, 2024
Short summary
Short summary
GEO4PALM is an open-source tool to generate static input for the Parallelized Large-Eddy Simulation (PALM) model system. Geospatial static input is essential for realistic PALM simulations. However, existing tools fail to generate PALM's geospatial static input for most regions. GEO4PALM is compatible with diverse geospatial data sources and provides access to free data sets. In addition, this paper presents two application examples, which show successful PALM simulations using GEO4PALM.
Piotr Zmijewski, Piotr Dziekan, and Hanna Pawlowska
Geosci. Model Dev., 17, 759–780, https://doi.org/10.5194/gmd-17-759-2024, https://doi.org/10.5194/gmd-17-759-2024, 2024
Short summary
Short summary
In computer simulations of clouds it is necessary to model the myriad of droplets that constitute a cloud. A popular method for this is to use so-called super-droplets (SDs), each representing many real droplets. It has remained a challenge to model collisions of SDs. We study how precipitation in a cumulus cloud depends on the number of SDs. Surprisingly, we do not find convergence in mean precipitation even for numbers of SDs much larger than typically used in simulations.
Roya Ghahreman, Wanmin Gong, Paul A. Makar, Alexandru Lupu, Amanda Cole, Kulbir Banwait, Colin Lee, and Ayodeji Akingunola
Geosci. Model Dev., 17, 685–707, https://doi.org/10.5194/gmd-17-685-2024, https://doi.org/10.5194/gmd-17-685-2024, 2024
Short summary
Short summary
The article explores the impact of different representations of below-cloud scavenging on model biases. A new scavenging scheme and precipitation-phase partitioning improve the model's performance, with better SO42- scavenging and wet deposition of NO3- and NH4+.
Daisuke Goto, Tatsuya Seiki, Kentaroh Suzuki, Hisashi Yashiro, and Toshihiko Takemura
Geosci. Model Dev., 17, 651–684, https://doi.org/10.5194/gmd-17-651-2024, https://doi.org/10.5194/gmd-17-651-2024, 2024
Short summary
Short summary
Global climate models with coarse grid sizes include uncertainties about the processes in aerosol–cloud–precipitation interactions. To reduce these uncertainties, here we performed numerical simulations using a new version of our global aerosol transport model with a finer grid size over a longer period than in our previous study. As a result, we found that the cloud microphysics module influences the aerosol distributions through both aerosol wet deposition and aerosol–cloud interactions.
Alexander de Meij, Cornelis Cuvelier, Philippe Thunis, Enrico Pisoni, and Bertrand Bessagnet
Geosci. Model Dev., 17, 587–606, https://doi.org/10.5194/gmd-17-587-2024, https://doi.org/10.5194/gmd-17-587-2024, 2024
Short summary
Short summary
In our study the robustness of the model responses to emission reductions in the EU is assessed when the emission data are changed. Our findings are particularly important to better understand the uncertainties associated to the emission inventories and how these uncertainties impact the level of accuracy of the resulting air quality modelling, which is a key for designing air quality plans. Also crucial is the choice of indicator to avoid misleading interpretations of the results.
Haiqin Li, Georg A. Grell, Ravan Ahmadov, Li Zhang, Shan Sun, Jordan Schnell, and Ning Wang
Geosci. Model Dev., 17, 607–619, https://doi.org/10.5194/gmd-17-607-2024, https://doi.org/10.5194/gmd-17-607-2024, 2024
Short summary
Short summary
We developed a simple and realistic method to provide aerosol emissions for aerosol-aware microphysics in a numerical weather forecast model. The cloud-radiation differences between the experimental (EXP) and control (CTL) experiments responded to the aerosol differences. The strong positive precipitation biases over North America and Europe from the CTL run were significantly reduced in the EXP run. This study shows that a realistic representation of aerosol emissions should be considered.
Giancarlo Ciarelli, Sara Tahvonen, Arineh Cholakian, Manuel Bettineschi, Bruno Vitali, Tuukka Petäjä, and Federico Bianchi
Geosci. Model Dev., 17, 545–565, https://doi.org/10.5194/gmd-17-545-2024, https://doi.org/10.5194/gmd-17-545-2024, 2024
Short summary
Short summary
The terrestrial ecosystem releases large quantities of biogenic gases in the Earth's Atmosphere. These gases can effectively be converted into so-called biogenic aerosol particles and, eventually, affect the Earth's climate. Climate prediction varies greatly depending on how these processes are represented in model simulations. In this study, we present a detailed model evaluation analysis aimed at understanding the main source of uncertainty in predicting the formation of biogenic aerosols.
Jiachen Liu, Eric Chen, and Shannon L. Capps
Geosci. Model Dev., 17, 567–585, https://doi.org/10.5194/gmd-17-567-2024, https://doi.org/10.5194/gmd-17-567-2024, 2024
Short summary
Short summary
Air pollution harms human life and ecosystems, but its sources are complex. Scientists and policy makers use air pollution models to advance knowledge and inform control strategies. We implemented a recently developed numeral system to relate any set of model inputs, like pollutant emissions from a given activity, to all model outputs, like concentrations of pollutants harming human health. This approach will be straightforward to update when scientists discover new processes in the atmosphere.
Gerrit Kuhlmann, Erik F. M. Koene, Sandro Meier, Diego Santaren, Grégoire Broquet, Frédéric Chevallier, Janne Hakkarainen, Janne Nurmela, Laia Amorós, Johanna Tamminen, and Dominik Brunner
EGUsphere, https://doi.org/10.5194/egusphere-2023-2936, https://doi.org/10.5194/egusphere-2023-2936, 2024
Short summary
Short summary
We present a Python software library for data-driven emission quantification (ddeq). It can be used to determine the emissions of hot spots (cities, power plants and industry) from remote sensing images using different methods. ddeq can be extended for new datasets and methods, providing a powerful community tool for users and developers. The application of the methods is shown using Jupyter Notebooks included in the library.
Kun Zheng, Qiya Tan, Huihua Ruan, Jinbiao Zhang, Cong Luo, Siyu Tang, Yunlei Yi, Yugang Tian, and Jianmei Cheng
Geosci. Model Dev., 17, 399–413, https://doi.org/10.5194/gmd-17-399-2024, https://doi.org/10.5194/gmd-17-399-2024, 2024
Short summary
Short summary
Radar echo extrapolation is the common method in precipitation nowcasting. Deep learning has potential in extrapolation. However, the existing models have low prediction accuracy for heavy rainfall. In this study, the prediction accuracy is improved by suppressing the blurring effect of rain distribution and reducing the negative bias. The results show that our model has better performance, which is useful for urban operation and flood prevention.
Li Pan, Partha S. Bhattacharjee, Li Zhang, Raffaele Montuoro, Barry Baker, Jeff McQueen, Georg A. Grell, Stuart A. McKeen, Shobha Kondragunta, Xiaoyang Zhang, Gregory J. Frost, Fanglin Yang, and Ivanka Stajner
Geosci. Model Dev., 17, 431–447, https://doi.org/10.5194/gmd-17-431-2024, https://doi.org/10.5194/gmd-17-431-2024, 2024
Short summary
Short summary
A GEFS-Aerosols simulation was conducted from 1 September 2019 to 30 September 2020 to evaluate the model performance of GEFS-Aerosols. The purpose of this study was to understand how aerosol chemical and physical processes affect ambient aerosol concentrations by placing aerosol wet deposition, dry deposition, reactions, gravitational deposition, and emissions into the aerosol mass balance equation.
Sean Raffuse, Susan O'Neill, and Rebecca Schmidt
Geosci. Model Dev., 17, 381–397, https://doi.org/10.5194/gmd-17-381-2024, https://doi.org/10.5194/gmd-17-381-2024, 2024
Short summary
Short summary
Large wildfires are increasing throughout the western United States, and wildfire smoke is hazardous to public health. We developed a suite of tools called rapidfire for estimating particle pollution during wildfires using routinely available data sets. rapidfire uses official air monitoring, satellite data, meteorology, smoke modeling, and low-cost sensors. Estimates from rapidfire compare well with ground monitors and are being used in public health studies across California.
Manuel F. Schmid, Marco G. Giometto, Gregory A. Lawrence, and Marc B. Parlange
Geosci. Model Dev., 17, 321–333, https://doi.org/10.5194/gmd-17-321-2024, https://doi.org/10.5194/gmd-17-321-2024, 2024
Short summary
Short summary
Turbulence-resolving flow models have strict performance requirements, as simulations often run for weeks using hundreds of processes. Many flow scenarios also require the flexibility to modify physical and numerical models for problem-specific requirements. With a new code written in Julia we hope to make such adaptations easier without compromising on performance. In this paper we discuss the modeling approach and present validation and performance results.
Yafang Guo, Chayan Roychoudhury, Mohammad Amin Mirrezaei, Rajesh Kumar, Armin Sorooshian, and Avelino F. Arellano
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2023-234, https://doi.org/10.5194/gmd-2023-234, 2024
Revised manuscript accepted for GMD
Short summary
Short summary
This research focuses on surface ozone (O3) pollution in Arizona, a historically air quality-challenged arid/semi-arid region in the US. The unique characteristics of semi-arid/arid regions, e.g., intense heat, minimal moisture, persistent desert shrubs, play a vital role in comprehending O3 exceedances. Using the WRF-Chem model, we analyzed O3 levels in the pre-monsoon month, revealing the model's skill in capturing diurnal and MDA8 O3 levels.
Marie-Noëlle Bouin, Cindy Lebeaupin Brossier, Sylvie Malardel, Aurore Voldoire, and César Sauvage
Geosci. Model Dev., 17, 117–141, https://doi.org/10.5194/gmd-17-117-2024, https://doi.org/10.5194/gmd-17-117-2024, 2024
Short summary
Short summary
In numerical models, the turbulent exchanges of heat and momentum at the air–sea interface are not represented explicitly but with parameterisations depending on the surface parameters. A new parameterisation of turbulent fluxes (WASP) has been implemented in the surface model SURFEX v8.1 and validated on four case studies. It combines a close fit to observations including cyclonic winds, a dependency on the wave growth rate, and the possibility of being used in atmosphere–wave coupled models.
Michal Belda, Nina Benešová, Jaroslav Resler, Peter Huszár, Ondřej Vlček, Pavel Krč, Jan Karlický, Pavel Juruš, and Kryštof Eben
EGUsphere, https://doi.org/10.5194/egusphere-2023-2740, https://doi.org/10.5194/egusphere-2023-2740, 2024
Short summary
Short summary
For modeling atmospheric chemistry, it is necessary to provide data on emissions of pollutants. These can come from various sources and in various forms and preprocessing of the data to be ingestible by chemistry models can be quite challenging. We developed the FUME processor to use a database layer that internally transforms all input data into a rigid structure facilitating further processing to allow emission processing from continental to street scale.
Najmeh Kaffashzadeh and Abbas Ali Aliakbari Bidokhti
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2023-226, https://doi.org/10.5194/gmd-2023-226, 2024
Revised manuscript accepted for GMD
Short summary
Short summary
Reanalysis data have been widely used as an initial condition for the daily forecast of the atmosphere or boundary conditions in regional models, for the study of climate change, and as proxies to complement insufficient in situ measurements. This paper assesses the capability of two state-of-the-art global datasets in simulating surface ozone over Iran using a new methodology.
Zehua Bai, Qizhong Wu, Kai Cao, Yiming Sun, and Huaqiong Cheng
EGUsphere, https://doi.org/10.5194/egusphere-2023-2962, https://doi.org/10.5194/egusphere-2023-2962, 2024
Short summary
Short summary
There are relatively limited researches on the application of scientific computing on RISC CPU platforms. The MIPS architecture CPUs, a type of RISC CPU, have distinct advantages in energy efficiency and scalability. In this study, the air quality modeling system can run stably on MIPS CPU platform, and the experiment results verify the stability of scientific computing on the platform. The work provides a technical foundation for the scientific application based on MIPS CPU platforms.
Lukas Fehr, Chris McLinden, Debora Griffin, Daniel Zawada, Doug Degenstein, and Adam Bourassa
Geosci. Model Dev., 16, 7491–7507, https://doi.org/10.5194/gmd-16-7491-2023, https://doi.org/10.5194/gmd-16-7491-2023, 2023
Short summary
Short summary
This work highlights upgrades to SASKTRAN, a model that simulates sunlight interacting with the atmosphere to help measure trace gases. The upgrades were verified by detailed comparisons between different numerical methods. A case study was performed using SASKTRAN’s multidimensional capabilities, which found that ignoring horizontal variation in the atmosphere (a common practice in the field) can introduce non-negligible errors where there is snow or high pollution.
Sylvain Mailler, Romain Pennel, Laurent Menut, and Arineh Cholakian
Geosci. Model Dev., 16, 7509–7526, https://doi.org/10.5194/gmd-16-7509-2023, https://doi.org/10.5194/gmd-16-7509-2023, 2023
Short summary
Short summary
We show that a new advection scheme named PPM + W (piecewise parabolic method + Walcek) offers geoscientific modellers an alternative, high-performance scheme designed for Cartesian-grid advection, with improved performance over the classical PPM scheme. The computational cost of PPM + W is not higher than that of PPM. With improved accuracy and controlled computational cost, this new scheme may find applications in chemistry-transport models, ocean models or atmospheric circulation models.
David R. Shaw, Toby J. Carter, Helen L. Davies, Ellen Harding-Smith, Elliott C. Crocker, Georgia Beel, Zixu Wang, and Nicola Carslaw
Geosci. Model Dev., 16, 7411–7431, https://doi.org/10.5194/gmd-16-7411-2023, https://doi.org/10.5194/gmd-16-7411-2023, 2023
Short summary
Short summary
Exposure to air pollution is one of the greatest risks to human health, and it is indoors, where we spend upwards of 90 % of our time, that our exposure is greatest. The INdoor CHEMical model in Python (INCHEM-Py) is a new, community-led box model that tracks the evolution and fate of atmospheric chemical pollutants indoors. We have shown the processes simulated by INCHEM-Py, its ability to model experimental data and how it may be used to develop further understanding of indoor air chemistry.
Willem E. van Caspel, David Simpson, Jan Eiof Jonson, Anna M. K. Benedictow, Yao Ge, Alcide di Sarra, Giandomenico Pace, Massimo Vieno, Hannah L. Walker, and Mathew R. Heal
Geosci. Model Dev., 16, 7433–7459, https://doi.org/10.5194/gmd-16-7433-2023, https://doi.org/10.5194/gmd-16-7433-2023, 2023
Short summary
Short summary
Radiation coming from the sun is essential to atmospheric chemistry, driving the breakup, or photodissociation, of atmospheric molecules. This in turn affects the chemical composition and reactivity of the atmosphere. The representation of photodissociation effects is therefore essential in atmospheric chemistry modeling. One such model is the EMEP MSC-W model, for which a new way of calculating the photodissociation rates is tested and evaluated in this paper.
Jungmin Lee, Walter M. Hannah, and David C. Bader
Geosci. Model Dev., 16, 7275–7287, https://doi.org/10.5194/gmd-16-7275-2023, https://doi.org/10.5194/gmd-16-7275-2023, 2023
Short summary
Short summary
Representing accurate land–atmosphere interaction processes is overlooked in weather and climate models. In this study, we propose three methods to represent land–atmosphere coupling in the Energy Exascale Earth System Model (E3SM) with the Multi-scale Modeling Framework (MMF) approach. In this study, we introduce spatially homogeneous and heterogeneous land–atmosphere interaction processes within the cloud-resolving model domain. Our 5-year simulations reveal only small differences.
Laurent Menut, Bertrand Bessagnet, Arineh Cholakian, Guillaume Siour, Sylvain Mailler, and Romain Pennel
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2023-209, https://doi.org/10.5194/gmd-2023-209, 2023
Revised manuscript accepted for GMD
Short summary
Short summary
This study is about the modelling of the atmospheric composition in Europe and during the summer 2022, when massive wildfires were observed. It is a sensitivity study dedicated to the relative impact of two modelling processes able to modify the meteorology used for the calculation of the atmospheric chemistry and transport of pollutants.
Bing Zhang, Mingjian Zeng, Anning Huang, Zhengkun Qin, Couhua Liu, Wenru Shi, Xin Li, Kefeng Zhu, Chunlei Gu, and Jialing Zhou
EGUsphere, https://doi.org/10.5194/egusphere-2023-2613, https://doi.org/10.5194/egusphere-2023-2613, 2023
Short summary
Short summary
By directly analysing the proximity of precipitation forecasts and observations, a precipitation forecast accuracy score (PAS) method was constructed. This method does not utilize the traditional contingency table-based classification verification, can replace the threat score (TS), equitable threat score (ETS) and other skill score methods, and can be used to calculate the accuracy of numerical models or quantitative precipitation forecasts.
Cited articles
Ashmore, M. R. and Dimitripoulou, C.: Personal exposure of children to air pollution, Atmos. Environ., 43, 128–141, https://doi.org/10.1016/j.atmosenv.2008.09.024, 2009.
Beckx, C., Int Panis, L., Arentze, T., Janssens, D., Torfs, R., Broekx, S., and Wets, G.: A dynamic activity-based population modelling approach to evaluate exposure to air pollution: Methods and application to a Dutch urban area, Environ. Impact Assess., 29, 179–185, 2009.
Bennett, D., McKone, T., Evans, J., Nazaroff, W., Smith, K., Margni, M., Jolliet, O., and Smith, K. R.: Defining intake fraction, Environ. Sci. Technol. 36, 206A–211A, https://doi.org/10.1021/es0222770, 2002.
Borrego, C., Sá, E., Monteiro, A., Ferreira, J., and Miranda, A.: Forecasting Human Exposure to atmospheric Pollutants – A modelling approach, Atmos. Environ., 43, 5796–5806, https://doi.org/10.1016/j.atmosenv.2009.07.049, 2009.
City of Helsinki Urban Facts (CHUF): Statistical Yearbook of the City of Helsinki, Gummerrus Kirjapaino Oy, Jyväskylä, 2009.
Dimitroulopoulou, C., Ashmore, M. R., Hill, M. T. R., Byrne, M. A., and Kinnersley, R.: INDAIR: a probabilistic model of indoor air pollution in UK homes, Atmos. Environ., 40, 6362–6379, https://doi.org/10.1016/j.atmosenv.2006.05.047, 2006.
Elolähde, T.: Traffic model system and emission calculations of the Helsinki Metropolitan Area Council, 20th International Emme Users' Conference, Montreal, available at: www.inro.ca/en/pres_pap/international/ieug06/1-3_Timo_Elolahde_report.pdf (last access: 18 December 2013), 2006.
European Parliament (EP): Directive 2002/91/EC of the European Parliament and of the Council of 16 December 2002 on the Energy Performance of Buildings, available at: http://eur-lex.europa.eu/legal-content/EN/TXT/?uri=CELEX:32002L0091 (last access: 25 August 2014), 2002.
Franzen, L. G., Hjelmroos, M., Kallberg, P., Brorstrom-Lunden, E., Juntto, S., and Savolainen, A.-L.: The "yellow snow" episode of northern Fennoscandia, March 1991 – a case study of long-distance transport of soil, pollen and stable organic compounds, Atmos. Environ., 28, 3587–3604, 1994.
Gulliver J. and Briggs, D.: Time-space modelling of journey-time exposure to traffic-related air pollution using GIS, Environ. Res., 97, 10–95, https://doi.org/10.1016/j.envres.2004.05.002, 2005.
Gröndahl, T., Makkonen, J., Myllynen, M., Niemi, J., and Tuomi, S.: Tulisijojen käyttö ja päästöt pääkaupunkiseudun pientaloista (The use of residential fireplaces and their emissions in the Helsinki Metropolitan Area), Helsingin seudun ympäristöpalvelut -kuntayhtymä, HSY, Helsinki, 2013 (in Finnish).
Hänninen, O., Kruize, H., Lebret, E., and Jantunen, M.: EXPOLIS simulation model: PM2.5 application and comparison with measurements in Helsinki, J. Exp. Anal. Environ. Epidem., 13, 74–85, https://doi.org/10.1038/sj.jea.7500260, 2003.
Hänninen, O., Lebret, E., Ilacqua, V., Katsouyanni, K., Künzli, N., Sram, R., and Jantunen, M.: Infiltration of ambient PM2.5 and levels of indoor generated non-ETS PM2.5 in residences of four European cities, Atmos. Environ., 38, 6411–6423, https://doi.org/10.1016/j.atmosenv.2004.07.015, 2004.
Hänninen, O., Palonen, J., Tuomisto, J., Yli-Tuomi, T., Seppänen, O., and Jantunen, M. J.: Reduction potential of urban PM2.5 mortality risk using modern ventilation systems in buildings, Indoor Air, 15, 246–256, https://doi.org/10.1111/j.1600-0668.2005.00365.x, 2005.
Hänninen, O., Hoek, G., Mallone, S., Chellini, E., Katsouyanni, K., Kuenzli, N., Gariazzo, C., Cattani, G., Marconi, A., Molnár, P., Bellander, T., and Jantunen, M.: Seasonal patterns of outdoor PM infiltration into indoor environments: review and meta-analysis of available studies from different climatological zones in Europe, Air Qual. Atmos. Health., 4, 221–233, https://doi.org/10.1007/s11869-010-0076-5, 2011.
Hänninen, O., Sorjamaa, R., Lipponen, P., Cyrys, J., Lanki, T., and Pekkanen, J.: Aerosol-based modelling of infiltration of ambient PM2.5 and evaluation against population-based measurements in homes in Helsinki, Finland, J. Aerosol Sci., 66, 111–122, https://doi.org/10.1016/j.jaerosci.2013.08.004, 2013.
Hellén, H., Kukkonen, J., Kauhaniemi, M., Hakola, H., Laurila, T., and Pietarila, H.: Evaluation of atmospheric benzene concentrations in the Helsinki Metropolitan Area in 2000–2003 using diffusive sampling and atmospheric dispersion modelling, Atmos. Environ., 39, 4003–4014, https://doi.org/10.1016/j.atmosenv.2005.03.023, 2005.
Hellman, T.: Henkilöautojen Keskikuormitus Niemen Rajalla Helsingissä Vuonna 2012 (The average number of people in the personal cars in Helsinki year 2012), City of Helsinki, City Planning Department, Traffic Planning, Publications on Air Quality, 23, 2012 (in Finnish).
INRO: EMME/2 User's manual, INRO Consultants Inc., Montreal, Canada, 1994.
Jalkanen, J.-P., Brink, A., Kalli, J., Pettersson, H., Kukkonen, J., and Stipa, T.: A modelling system for the exhaust emissions of marine traffic and its application in the Baltic Sea area, Atmos. Chem. Phys., 9, 9209–9223, https://doi.org/10.5194/acp-9-9209-2009, 2009.
Jalkanen, J.-P., Johansson, L., Kukkonen, J., Brink, A., Kalli, J., and Stipa, T.: Extension of an assessment model of ship traffic exhaust emissions for particulate matter and carbon monoxide, Atmos. Chem. Phys., 12, 2641–2659, https://doi.org/10.5194/acp-12-2641-2012, 2012.
Jantunen, M., Hänninen, O., Katsouyanni, K., Knöppel, H., Künzli, N., and Lebret, E.: Air pollution exposure in European cities: The EXPOLIS-study, J. Expo. Anal. Env. Epid., 8, 495–518, 1998.
Jensen, S. S.: A Geographic Approach to Modelling Human Exposure to Traffic Air Pollution using GIS, PhD Thesis. National Environ. Res. Institute, Denmark, 1999.
Kauhaniemi, M., Karppinen, A., Härkönen, J., Kousa, A., Alaviippola, B., Koskentalo, T., Aarnio, P., Elolähde, T., and Kukkonen, J.: Evaluation of a modelling system for predicting the concentrations of PM2.5 in an urban area, Atmos. Environ. 42, 4517–4529, https://doi.org/10.1016/j.atmosenv.2008.01.071, 2008.
Kauhaniemi, M., Kukkonen, J., Härkönen, J., Nikmo, J., Kangas, L., Omstedt, G., Ketzel, M., Kousa, A., Haakana, M., and Karppinen, A.: Evaluation of a road dust suspension model for predicting the concentrations of PM10 in a street canyon, Atmos. Environ., 45, 3646–3654, https://doi.org/10.1016/j.atmosenv.2011.04.055, 2011.
Karppinen, A.: Meteorological pre-processing and atmospheric dispersion modelling of urban air quality and applications in the Helsinki Metropolitan Area. Finnish Meteorological Institute, Contributions No. 33, ISBN 951-697-552-6, University Press, Helsinki, 2001.
Karppinen, A., Kukkonen, J., Elolähde, T., Konttinen, M., Koskentalo, T., and Rantakrans, E.: A modelling system for predicting urban air pollution, Model description and applications in the Helsinki Metropolitan Area, Atmos. Environ., 34, 3723–3733, https://doi.org/10.1016/S1352-2310(00)00074-1, 2000a.
Karppinen, A., Kukkonen, J., Elolähde, T., Konttinen, M., and Koskentalo, T.: A modelling system for predicting urban air pollution, Comparison of model predictions with the data of an urban measurement network, Atmos. Environ., 34, 3735–3743, https://doi.org/10.1016/S1352-2310(00)00073-X, 2000b.
Kousa, A., Kukkonen, J., Karppinen, A., Aarnio, P., and Koskentalo, T.: Statistical and diagnostic evaluation of a new-generation urban dispersion modelling system against an extensive dataset in the Helsinki Area, Atmos. Environ., 35, 4617–4628, https://doi.org/10.1016/S1352-2310(01)00163-7, 2001.
Kousa, A., Kukkonen, J., Karppinen, A., Aarnio, P., and Koskentalo, T.: A model for evaluating the population exposure to ambient air pollution in an urban area, Atmos. Environ., 36, 2109–2119, https://doi.org/10.1016/S1352-2310(02)00228-5, 2002.
Kukkonen, J., Härkönen, J., Walden, J., Karppinen, A., and Lusa, K.: Evaluation of the dispersion model CAR-FMI against data from a measurement campaign near a major road, Int. J. Environ. Pollut., 35, 949–960, 2001.
Lanki, T., Hoek, G., Timonen, K. L., Peters, A., Tiittanen, P., and Vanninen, E.: Hourly variation in fine particle exposure is associated with transiently increased risk of ST segment depression, Occup. Environ. Med., 65, 782–786, https://doi.org/10.1136/oem.2007.037531, 2008.
Lappi, S., Lovén, K., Rasila, T., and Pietarila, H.: Pääkaupunkiseudun päästöjen leviämismalliselvitys. Energiantuotannon, satamatoiminnan, laivaliikenteen, lentoliikenteen, lentoasematoiminnan ja autoliikenteen typenoksidi-, rikkidioksidi- ja hiukkaspäästöjen leviämislaskelmat, Finnish Meteorological Institute, Helsinki, 2008.
Laurikko, J.: On exhaust emissions from petrol-fuelled passenger cars at low ambient temperatures, VTT Publications 348, Technical Research Centre of Finland, Espoo, 210 pp., 1998.
Laurikko, J., Kukkonen, J., Koistinen, K., and Koskentalo, T.: Integrated modelling system for the evaluation of the impact of Transport-related measures to urban air quality, 2th symposium "Transport and Air Pollution", Avignon, France, 2003.
Levitin, J., Härkönen, J., Kukkonen, J., and Nikmo, J.: Evaluation of the CALINE4 and CAR-FMI models against measurements near a major road, Atmos. Environ., 39, 4439–4452, https://doi.org/10.1016/j.atmosenv.2005.03.046, 2005.
Loh, M. M., Soares, J., Karppinen, A., Kukkonen, J., Kangas, L., Riikonen, K., Kousa, A., Asikainen, A., and Jantunen, M. J.: Intake fraction distributions for benzene from vehicles in the Helsinki Metropolitan Area, Atmos. Environ., 43, 301–310, https://doi.org/10.1016/j.atmosenv.2008.09.082, 2009.
Mäkelä, K.: "LIPASTO calculation model: unit emissions of traffic", VTT Technical Research Centre of Finland, Espoo, Finland, available at: http://lipasto.vtt.fi/info.htm (last access: 9 April 2014), 2002.
Official Statistics of Finland (OSF): Time use survey [e-publication], Helsinki: Statistics Finland, available at: http://www.stat.fi/til/akay/index_en.html, last access: 1 January 2013.
Niemi, J., Malkki, M., Myllynen, M., Lounasheimo, J., Kousa, A., Julkunen, A., and Koskentalo, T.: Air Quality in the Helsinki Metropolitan Area in 2008, YTV Publications 15/2009, 128, Finland, available at: http://www.hsy.fi/seututieto/Documents/YTV_julkaisusarja/15_2009_vuosiraportti2008.pdf (last access: 12 June 2014), 2009 (in Finnish)
Omstedt, G., Bringfelt, B., and Johansson, C.: A model for vehicle-induced non-tailpipe emissions of particles along Swedish roads, Atmos. Environ., 39, 6088–6097, https://doi.org/10.1016/j.atmosenv.2005.06.037, 2005.
Öttl, D., Kukkonen, J., Almbauer, R. A., Sturm, P. J., Pohjola, M., and Härkönen, J. H.: Evaluation of a Gaussian and a Lagrangian model against a roadside dataset, with focus on low wind speed conditions, Atmos. Environ., 35, 2123–2132, https://doi.org/10.1016/S1352-2310(00)00492-1, 2001.
Pope, C. A. and Dockery, D. W.: Health effects of fine particulate air pollution: Lines that connect, J. Air Waste Manage., 56, 709–742, 2006.
Rotko, T., Koistinen, K., Hänninen, O., and Jantunen, M.: Sociodemographic descriptors of personal exposure to fine particles (PM2.5) in EXPOLIS Helsinki, J. Expo. Anal. Env. Epid., 10, 385–393, https://doi.org/10.1038/sj.jea.7500104, 2000.
Schaap, M. F. S., Timmermans, R. M. A., Roemer, M., Velders, G., Beck, J., and Builtjes, P. J. H.: The LOTOS-EUROS model: description, validation and latest developments, Int. J. Environ. Pollut., 32, 270–290, 2008.
Schweizer, C., Edwards, R. D, Bayer-Oglesby, L., Gauderman, W. J., Ilacqua, V., Juhani, M., Lai, H. K., Nieuwenhuijsen, M., and Künzl, N.: Indoor time-microenvironment-activity patterns in seven regions of Europe, J. Expo. Sci. Env. Epid., 17, 170–181, https://doi.org/10.1038/sj.jes.7500490, 2007.
Singh, V., Sokhi, R., and Kukkonen, J.: PM2.5 concentrations in London for 2008 – A modeling analysis of contributions from road traffic, J. Air Waste Manage., 64, 509–518, https://doi.org/10.1080/10962247.2013.848244, 2014.
Sofiev, M., Soares, J., Prank, M., de Leeuw, G., and Kukkonen, J.: A regional-to-global model of emission and transport of sea salt particles in the atmosphere, J. Geophys. Res., 116, D21302, https://doi.org/10.1029/2010JD014713, 2011.
Sokhi, R., Mao, H., Srimath, S. T. G., Fan, S., Kitwiroon, N., Luhana, L., Kukkonen, K., Haakana, M., van den Hout, K. D., Boulter, P., McCrae, I. S., Larssen, S., Gjerstad, K. I., San Jose, R., Bartzis, J., Neofytou, P., van den Breemer, P., Neville, S., Kousa, A., Cortes, B. M., Karppinen, K., and Myrtveit, I.: An integrated multi-model approach for air quality assessment: Development and evaluation of the OSCAR Air Quality Assessment System, Environ. Modell. Softw., 23, 268–281, https://doi.org/10.1016/j.envsoft.2007.03.006, 2008.
Statistics Filand: Energy consumption in households [e-publication], ISSN = 2323-329X, 2012, Appendix Figure 1, Energy consumption in households by energy source in 2012, Helsinki: Statistics Finland, available at: http://www.stat.fi/til/asen/2012/asen_2012_2013-11-13_kuv_001_en.html (last access: 30 June 2014), 2012.