Journal cover Journal topic
Geoscientific Model Development An interactive open-access journal of the European Geosciences Union
Geosci. Model Dev., 8, 975-1003, 2015
https://doi.org/10.5194/gmd-8-975-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
Model description paper
07 Apr 2015
Tropospheric chemistry in the Integrated Forecasting System of ECMWF
J. Flemming1, V. Huijnen2, J. Arteta3, P. Bechtold1, A. Beljaars1, A.-M. Blechschmidt4, M. Diamantakis1, R. J. Engelen1, A. Gaudel5, A. Inness1, L. Jones1, B. Josse3, E. Katragkou6, V. Marecal3, V.-H. Peuch1, A. Richter4, M. G. Schultz7, O. Stein7, and A. Tsikerdekis6 1European Centre for Medium-Range Weather Forecasts, Reading, UK
2Royal Netherlands Meteorological Institute, De Belt, the Netherlands
3Météo-France, Toulouse, France
4Universität Bremen, Bremen, Germany
5CNRS, Laboratoire d'Aérologie, UMR 5560, Toulouse, France
6Department of Meteorology and Climatology, School of Geology, Aristotle University of Thessaloniki, Thessaloniki, Greece
7Institute for Energy and Climate Research, Forschungszentrum Jülich, Jülich, Germany
Abstract. A representation of atmospheric chemistry has been included in the Integrated Forecasting System (IFS) of the European Centre for Medium-Range Weather Forecasts (ECMWF). The new chemistry modules complement the aerosol modules of the IFS for atmospheric composition, which is named C-IFS. C-IFS for chemistry supersedes a coupled system in which chemical transport model (CTM) Model for OZone and Related chemical Tracers 3 was two-way coupled to the IFS (IFS-MOZART). This paper contains a description of the new on-line implementation, an evaluation with observations and a comparison of the performance of C-IFS with MOZART and with a re-analysis of atmospheric composition produced by IFS-MOZART within the Monitoring Atmospheric Composition and Climate (MACC) project. The chemical mechanism of C-IFS is an extended version of the Carbon Bond 2005 (CB05) chemical mechanism as implemented in CTM Transport Model 5 (TM5). CB05 describes tropospheric chemistry with 54 species and 126 reactions. Wet deposition and lightning nitrogen monoxide (NO) emissions are modelled in C-IFS using the detailed input of the IFS physics package. A 1 year simulation by C-IFS, MOZART and the MACC re-analysis is evaluated against ozonesondes, carbon monoxide (CO) aircraft profiles, European surface observations of ozone (O3), CO, sulfur dioxide (SO2) and nitrogen dioxide (NO2) as well as satellite retrievals of CO, tropospheric NO2 and formaldehyde. Anthropogenic emissions from the MACC/CityZen (MACCity) inventory and biomass burning emissions from the Global Fire Assimilation System (GFAS) data set were used in the simulations by both C-IFS and MOZART. C-IFS (CB05) showed an improved performance with respect to MOZART for CO, upper tropospheric O3, and wintertime SO2, and was of a similar accuracy for other evaluated species. C-IFS (CB05) is about 10 times more computationally efficient than IFS-MOZART.

Citation: Flemming, J., Huijnen, V., Arteta, J., Bechtold, P., Beljaars, A., Blechschmidt, A.-M., Diamantakis, M., Engelen, R. J., Gaudel, A., Inness, A., Jones, L., Josse, B., Katragkou, E., Marecal, V., Peuch, V.-H., Richter, A., Schultz, M. G., Stein, O., and Tsikerdekis, A.: Tropospheric chemistry in the Integrated Forecasting System of ECMWF, Geosci. Model Dev., 8, 975-1003, https://doi.org/10.5194/gmd-8-975-2015, 2015.
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Short summary
We describe modules for atmospheric chemistry, wet and dry deposition and lightning NO production, which have been newly introduced in ECMWF's weather forecasting model. With that model, we want to forecast global air pollution as part of the European Copernicus Atmosphere Monitoring Service. We show that the new model results compare as well or better with in situ and satellite observations of ozone, CO, NO2, SO2 and formaldehyde as the previous model.
We describe modules for atmospheric chemistry, wet and dry deposition and lightning NO...
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